研究目的
研究缺陷与无金属掺杂在超薄二维材料中的协同效应,用于环境修复,特别是可见光照射下无色有机污染物的降解。
研究成果
富含氧空位的超薄硫掺杂BiOBr纳米片(BB-xS)在可见光下对无色有机污染物展现出优异的光催化降解活性,这归因于硫掺杂与氧空位的协同效应。该研究为设计高效环境修复光催化剂提供了新思路。
研究不足
该研究聚焦于特定无色有机污染物的降解,可能未涵盖所有类型的污染物。其在实际环境修复中的可扩展性和实际应用尚需进一步研究。
1:实验设计与方法选择:
采用一步溶剂热法合成了富氧空位超薄硫掺杂BiOBr纳米片(BB-xS)。
2:样品选择与数据来源:
选择无可见光吸收且存在于废水中的4-氯酚(4-CP)作为探针污染物。
3:实验设备与材料清单:
使用五水合硝酸铋、溴化钠、硫脲、聚乙烯吡咯烷酮(PVP,K-30)、甘油等化学品。
4:0)、甘油等化学品。 实验步骤与操作流程:
4. 实验步骤与操作流程:将Bi(NO3)3?5H2O和PVP分散于水和甘油的混合液中,加入NaBr和硫脲溶液,在聚四氟乙烯内衬的高压釜中加热。
5:数据分析方法:
通过可见光照射下4-CP的降解效率评估光催化活性,利用UPLC-MS分析中间产物,ESR检测活性自由基。
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X-ray diffractometer
Bruker D8
Bruker
Phase and crystallinity determination
-
SEM
Quanta 200FEG
FEI
Morphology and microstructure study
-
TEM
FEI Tecnai G2 F30
FEI
Morphology and microstructure study
-
TOC measuring instrument
Shimadz TOC-5000
Shimadzu
Analysis of total organic carbon concentrations
-
X-ray photoelectron spectroscopy
Thermo ESCALAB 250
Thermo
Chemical composition analysis
-
ESR spectroscopy
Bruker A300 spectrometer
Bruker
Investigation of oxygen vacancies and reactive radicals
-
UV–vis diffuse reflectance spectra
UV2550
Shimadzu
Optical properties evaluation
-
Photoluminescence spectra
F-4600
Hitachi
Study of photoexcited charge transfer behaviors
-
Short-arc xenon lamp
PE300BF
Perkin-Elmer
Light source for photocatalytic activity measurement
-
Bismuth nitrate pentahydrate
Bi(NO3)3?5H2O
Sinopharm Chemical Reagent Co. Ltd
Precursor for synthesizing BiOBr nanosheets
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Sodium bromide
NaBr
Sinopharm Chemical Reagent Co. Ltd
Source of bromine for BiOBr synthesis
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Thiourea
Sinopharm Chemical Reagent Co. Ltd
Sulfur source for doping
-
Polyvinylpyrrolidone
PVP, K-30
Sinopharm Chemical Reagent Co. Ltd
Stabilizer in the synthesis process
-
Glycerol
Sinopharm Chemical Reagent Co. Ltd
Solvent in the synthesis process
-
4-chlorophenol
4-CP
Sinopharm Chemical Reagent Co. Ltd
Probe contaminant for photocatalytic degradation
-
5,5-dimethyl-1-pyrroline N-oxide
DMPO
Sinopharm Chemical Reagent Co. Ltd
Spin trap for ESR spectroscopy
-
Bisphenol A
BPA
Sinopharm Chemical Reagent Co. Ltd
Colorless organic contaminant for degradation
-
Sulfadiazine
SDZ
Sinopharm Chemical Reagent Co. Ltd
Colorless organic contaminant for degradation
-
Sulfamerazine
SMZ
Sinopharm Chemical Reagent Co. Ltd
Colorless organic contaminant for degradation
-
Methanol
Sinopharm Chemical Reagent Co. Ltd
Solvent
-
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