摘要： When a graphene ?lm is coated onto a ?exible polymer substrate, weak adhesion can cause delamination of the ?lm under mechanical bending. Moreover, as each graphene layer restacks, the performance of the ?lm as an electrode for a supercapacitor becomes limited. In this study, facile laser welding and surface modi?cation processes are demonstrated to overcome these limitations. First, a continuous wave laser beam is applied to the interface between the coated graphene and the underlying transparent polycarbonate substrate. This welding process signi?cantly improves their adhesion and enables excellent mechanical bendability. Second, surface modi?cation of graphene is achieved under ambient conditions by irradiating the graphene ?lm surface with a nanosecond pulsed laser. Sandwich-type supercapacitors are fabricated using these surface-modi?ed graphene electrodes with a PVA-H3PO4 electrolyte. The e?ect of the laser ?uence on the performance of the supercapacitor is investigated. At an optimal laser power, an areal capacitance of 4.7 mF/cm2 is achieved.