研究目的
Understanding the contrast mechanism in second harmonic microscopy of poled x-cut thin film lithium niobate for both fundamental physics and device developments.
研究成果
The study concludes that second-harmonic microscopy can unambiguously distinguish between completely and partly inverted domains in thin film lithium niobate, providing a noninvasive tool for analyzing ferroelectric domain structures. The depth of poling can be determined with tens of nanometers resolution, which is crucial for device development.
研究不足
The study is limited by the diffraction-limited resolution of the microscope and the influence of interfacial reflections and resonant enhancements on the SH signal. The model assumes an extensionless transition for domain walls, which may not account for all real-world complexities.
1:Experimental Design and Method Selection:
The study employs second-harmonic microscopy to visualize and analyze ferroelectric domain structures in thin film lithium niobate. The methodology includes a full three-dimensional focus calculation accounting for interface reflections.
2:Sample Selection and Data Sources:
The samples are x-cut lithium niobate thin films on silicon handles with a buried oxide layer. Data is acquired through SH microscopy.
3:List of Experimental Equipment and Materials:
A femtosecond mode-locked Ti:Sapphire laser is used as the pump source. Microscope objectives with different numerical apertures are employed for focusing. The SH light is detected using a silicon single photon avalanche diode.
4:Experimental Procedures and Operational Workflow:
The pump light is focused onto the sample, and the generated SH light is collected in the backward direction. The sample is raster-scanned to generate images.
5:Data Analysis Methods:
The SH signal is analyzed based on phase matching, interface reflections, and resonant enhancements. Simulations are performed to understand the effects of these parameters on the SH signal.
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