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Fabrication and characterization of microcavity organic light-emitting diode with CaF2/ZnS distributed Bragg reflector

DOI:10.1016/j.tsf.2020.137912 期刊:Thin Solid Films 出版年份:2020 更新时间:2025-09-19 17:13:59
摘要: We fabricated alternately multilayered films using CaF2 and ZnS with a different number of pairs by thermal evaporation method and evaluated their reflectance as a distributed Bragg reflector (DBR). A 7-pair CaF2/ZnS multilayered film had an enough high reflectance for use as DBR in the wavelength region of 400–600 nm, which is good agreement with the theoretically calculated reflectance. The fabricated CaF2/ZnS multilayered film was incorporated to the organic light-emitting diode (OLED) devices. We found that the inversed-type OLED (iOLED) structure is suitable for achieving the working device. From the result of electroluminescence (EL) measurement, the spectral linewidth of EL of inversed OLED with DBR (μ-cavity iOLED) was significantly narrowed compared to that of conventional OLED (cOLED). The EL peak wavelength of μ-cavity iOLED was centered around 520 nm, which was well corresponded to the designed cavity length. The observed narrowing of EL spectra for μ-cavity iOLED was originated from the microcavity effect. Color coordinate of the emission were changed from cOLED: (0.31, 0.54) to μ-cavity iOLED (0.20, 0.72), which indicates a significant improvement of color purity of green emission.
作者: Takuya Kitabayashi,Teruyuki Asashita,Naoya Satoh,Takayuki Kiba,Midori Kawamura,Yoshio Abe,Kyung Ho Kim
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Investigating the fabrication and characterization of microcavity organic light-emitting diodes (OLEDs) with CaF2/ZnS distributed Bragg reflectors (DBRs) to improve color purity.

The study successfully demonstrated the fabrication of CaF2/ZnS multilayered films with high reflectance suitable for use as DBRs in OLEDs. The incorporation of these DBRs into inverted OLED structures significantly improved the color purity of green emission through the microcavity effect. The method is compatible with any emissive material and offers a simple approach to enhancing OLED performance.

The study mentions the failure of standard OLED devices due to electrical short circuits caused by the roughness of the bottom DBR, leading to the adoption of an inverted OLED structure. The device performance, including current efficiency and luminance, was lower than that of conventional OLEDs.

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