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Reconstruction of attosecond pulses in the presence of interfering dressing fields using a 100 kHz laser system at ELI-ALPS

DOI:10.1088/1361-6455/ab486c 期刊:Journal of Physics B: Atomic, Molecular and Optical Physics 出版年份:2019 更新时间:2025-09-23 15:19:57
摘要: Attosecond Pulse Trains (APT) generated by high-harmonic generation (HHG) of high-intensity near-infrared (IR) laser pulses have proven valuable for studying the electronic dynamics of atomic and molecular species. However, the high intensities required for high-photon-energy, high-flux HHG usually limit the class of adequate laser systems to repetition rates below 10 kHz. Here, APT’s generated from the 100 kHz, 160 W, 40 fs laser system (HR-1) currently under commissioning at the Extreme Light Infrastructure Attosecond Light Pulse Source (ELI-ALPS) are reconstructed using the Reconstruction of Attosecond Beating By Interference of two-photon Transitions (RABBIT) technique. These experiments constitute the first attosecond time-resolved photoelectron spectroscopy measurements with attosecond pulses performed at 100 kHz repetition rate and one of the first experiments performed at ELI-ALPS in the framework of projects commissioning its newly installed technologies. These RABBIT measurements were taken with an additional IR field temporally locked to the extreme-ultraviolet APT, resulting in an atypical ω beating. We show that the phase of the 2ω beating recorded under these conditions is strictly identical to that observed in standard RABBIT measurements within second-order perturbation theory. This work highlights an experimental simplification for future experiments based on attosecond interferometry (or RABBIT), which is particularly useful when lasers with high average powers are used.
作者: Daniel Hammerland,P. Zhang,S. Kühn,P. Jojart,I. Seres,V. Zuba,Z. Varallyay,D. Charalambidis,K. Osvay,T. T. Luu,H. J. W?rner
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To reconstruct Attosecond Pulse Trains (APT) generated by high-harmonic generation (HHG) using a 100 kHz laser system at ELI-ALPS and to demonstrate the RABBIT technique in the presence of an additional IR field temporally locked to the APT.

The RABBIT technique was successfully tailored to work with an additional IR pulse temporally locked to the XUV APT, demonstrating identical information encoding as in standard RABBIT schemes. This method simplifies future attosecond pulse metrology and measurements of attosecond photoionization delays at high repetition rates and high average powers.

The high average power of the laser system posed challenges in managing thermal loads on optics and the fragility of metallic foils used for filtering XUV light. The inability to filter IR from XUV led to high average IR powers being incident on the XUV mirror, causing thermal expansion.

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