研究目的
Investigating the shrinkage dynamics of plasmonic bubbles formed around metallic nanoparticles immersed in liquid and irradiated by a resonant light source, focusing on the two different phases of shrinkage: rapid partial bubble shrinkage governed by vapor condensation and slow diffusion-controlled bubble dissolution.
研究成果
The study concludes that plasmonic bubble shrinkage involves two distinct phases: a rapid vapor condensation phase influenced by the bubble's formation history and a slow diffusion phase dependent on dissolved air concentration. A transition in scaling laws for bubble dissolution is observed with varying air concentrations, explained theoretically.
研究不足
The study is limited to specific conditions of laser power, pulse duration, and dissolved air concentrations. The initial temperature distribution in the liquid is uncertain, affecting the accuracy of model predictions during the transition between shrinkage phases.
1:Experimental Design and Method Selection:
The study involves the formation of plasmonic bubbles around metallic nanoparticles in liquid under laser irradiation, observing their shrinkage dynamics. Theoretical models are employed to explain the observed phenomena.
2:Sample Selection and Data Sources:
Gold nanoparticles on a fused-silica substrate immersed in water with varying dissolved air concentrations are used. Data is collected through high-speed imaging.
3:List of Experimental Equipment and Materials:
A continuous-wave laser, acousto-optic modulator, high-speed cameras, and an oxygen meter for measuring air concentration levels.
4:Experimental Procedures and Operational Workflow:
Laser pulses of varying power and duration are used to form bubbles, and their shrinkage is recorded after the laser is turned off.
5:Data Analysis Methods:
Image segmentation algorithms are used to extract bubble parameters, and theoretical models are compared with experimental data.
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