研究目的
To propose a technique called compressed ultrafast electron di?raction imaging (CUEDI) to overcome the technical limitations of ultrafast electron di?raction (UED), such as the requirement for highly repeatable measurements and the significant effect of relative time jitter between laser and electron pulses on temporal resolution.
研究成果
The CUEDI technique can provide a well-established tool to recover the time-evolving electron diffraction pattern with a single shot measurement, eliminating the relative time jitter between the pump-laser pulse and the probe electron pulse. This method shows great potential for replacing the traditional pump-probe scheme in the study of real-time structural dynamics.
研究不足
The temporal resolution for CUEDI is mainly limited by the kinetic energy dispersion of the electron source, the time-varying voltage in the deflection plate, and the distance between the deflection plate and CCD detector. Additionally, the electron beamlet expansion due to the space-charge effect (SCE) needs to be carefully managed.
1:Experimental Design and Method Selection:
The CUEDI technique involves encoding time-evolving electron di?raction patterns with random codes on an electron encoder, measuring the encoded pattern after a temporal shearing operation, and reconstructing the evolution process using a compressed sensing algorithm.
2:Sample Selection and Data Sources:
The feasibility of CUEDI is confirmed by numerically simulating the polycrystalline gold melting process based on experimental data measured with the pump-probe method.
3:List of Experimental Equipment and Materials:
Includes an electron encoder composed of randomly distributed microchannel tubes and micro-Faraday cups, a time-varying electric field for deflection, and a detector for recording the encoded electron diffraction pattern.
4:Experimental Procedures and Operational Workflow:
The electron beam is diffracted by the sample, encoded by the electron encoder, deflected by a time-varying electric field, and recorded by the detector. The time-evolving electron diffraction pattern is then reconstructed using a compressed sensing algorithm.
5:Data Analysis Methods:
A two-step iterative shrinkage/thresholding (TwIST) algorithm is employed to reconstruct the time-evolving electron diffraction pattern from the encoded and measured data.
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