研究目的
To characterize high harmonics from magnesium oxide and quartz crystals using an interferometric method and measure material-dependent intensity-induced high-harmonic phase delays.
研究成果
The material-dependent dipole phase can provide a robust platform for high-harmonic spectroscopy of solids. Measured phase shifts in the reflection geometry can be reproduced from the diabatic dipole moment of a strongly driven two-level system.
研究不足
The nonlinear refractive indices are often anisotropic, the spatiotemporal properties of high harmonics could depend on the crystal orientation in a non-trivial manner, in addition to their microscopic origin.
1:Experimental Design and Method Selection:
Employed an interferometric method to characterize high harmonics from magnesium oxide and quartz crystals.
2:Sample Selection and Data Sources:
Used 200-μm-thick MgO crystals and SiO2 crystals subjected to strong near-infrared laser pulses.
3:List of Experimental Equipment and Materials:
Optical parametric amplifier (OPA), Ti:sapphire amplifier, NIR interferometer, imaging spectrometer.
4:Experimental Procedures and Operational Workflow:
The laser beam was split into two using an interferometer and focused into two spatially separated spots on the sample. The high-harmonic beams generated from each focus overlapped in the far field. An imaging spectrometer was used to record the EUV spectrographs.
5:Data Analysis Methods:
Analyzed the relative phase shifts on individual harmonics through corresponding fringe shifts at various pump laser intensities and two wavelengths.
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