研究目的
Investigating the effects of two-center interference and molecular scattering phase in the transfer of linear photon momentum to the ionized electron by absorbing a single photon in diatomic molecules.
研究成果
The study demonstrates significant deviations from the prediction of the classical double-slit model due to the strong mediation of the Coulomb potential and shows that a varying molecular scattering phase is important at all electron energies, beyond the simple prediction of the linear combination of the atomical orbitals. The electric quadrupole term contributes dominantly to the linear photon momentum transfer for the molecule.
研究不足
The study is limited to the simplest diatomic molecule H2+ and does not account for the influence of the ground vibrational state to the oscillation feature of the transferred linear momentum of the electron in detail.
1:Experimental Design and Method Selection:
The time-dependent Schr?dinger equation of H2+ is numerically solved in the multipolar gauge to separate the contributions of the electric quadrupole term and the magnetic dipole term in the momentum transfer.
2:Sample Selection and Data Sources:
The study focuses on the simplest diatomic molecule H2+ as a benchmark system.
3:List of Experimental Equipment and Materials:
Not explicitly mentioned in the paper.
4:Experimental Procedures and Operational Workflow:
The transferred momentum to the electron is evaluated at different internuclear distances with various photon energies for different configurations of the molecular and the laser orientation.
5:Data Analysis Methods:
The average momentum of the photoelectron is evaluated by integrating over the photoelectron momentum distribution.
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