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Results from the validation campaign of the ozone radiometer GROMOS-C at the NDACC station of La Réunion Island

DOI:10.5194/acp-2016-117 期刊:Atmospheric Chemistry and Physics Discussions 出版年份:2016 更新时间:2025-09-23 15:23:52
摘要: Ozone is a species of primary interest as it performs a key role in the middle atmosphere and its monitoring is thus necessary. At the Institute of Applied Physics of the University of Bern, Switzerland, we built a new ground based microwave radiometer, GROMOS-C (GRound based Ozone MOnitoring System for Campaigns). It has a compact design and can be operated at remote places with very little maintenance requirements, being therefore suitable for remote deployments. It has been conceived to measure the vertical distribution of ozone in the middle atmosphere, by observing pressure broadened emission spectra at a frequency of 110.836 GHz. In addition, meridional and zonal wind profiles can be retrieved, based on the Doppler shift of the ozone line measured in the 4 directions of observation (North-East-South-West). In June 2014 the radiometer was installed in the Ma?do observatory, on La Réunion Island (21.2°S, 55.5°E). High resolution ozone spectra were continuously recorded during 7 months. Vertical profiles of ozone have been retrieved through an optimal estimation inversion process, using the Atmospheric Radiative Transfer Simulator ARTS2 as the forward model. The best estimate of the vertical profile is done by means of the optimal estimation method. The validation is performed against ozone profiles from the Microwave Limb Sounder (MLS) on the Aura satellite, the ozone lidar located in the observatory and with ozone profiles from weekly radiosondes. Zonal and meridional winds retrieved from GROMOS-C data are validated against another wind radiometer located in situ, WIRA. In addition, we compare both ozone and winds with ECMWF model data. Results show that GROMOS-C provides reliable ozone profiles between 30 to 0.02 hPa. The comparison with lidar shows a very good agreement at all levels. The accordance with MLS is within less than 10% for pressure levels between 25 and 0.2 hPa.
作者: Susana Fernandez,Rolf Rüfenacht,Niklaus K?mpfer,Thierry Portafaix,Fran?oise Posny,Guillaume Payen
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To validate the performance of the GROMOS-C radiometer for measuring ozone and wind profiles in the middle atmosphere by comparing it with other reliable instruments and models.

GROMOS-C is validated as a reliable instrument for continuous ozone profile measurements with high temporal resolution in the middle atmosphere (30 to 0.02 hPa), showing good agreement with MLS (within 10%), lidar (within 5%), and ECMWF models. It also demonstrates capability for wind profile retrieval, capturing key meteorological features. The multiple calibration methods provide flexibility under varying conditions. Future work should investigate the diurnal ozone cycle in tropical regions.

The retrieval reliability is limited to pressure levels between 30 and 0.02 hPa; below 30 hPa, discrepancies increase. High humidity conditions can cause calibration issues, such as baseline ripples from water condensation. The vertical resolution varies from 7 km to 17 km, which is coarser than some reference instruments. Wind measurements have larger uncertainties and a smaller altitude range compared to specialized instruments like WIRA.

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