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[IEEE 2019 Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC) - Munich, Germany (2019.6.23-2019.6.27)] 2019 Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC) - Toward Coupling Color Centers in Single Crystal Diamond to Two-Dimensional Materials
摘要: Individual nitrogen vacancy (NV) color centers in diamond are bright, photo-stable, atomic-sized dipole emitters [1]. Consequently, they represent optimal candidates for novel scanning near field microscopy techniques [2]. Here, NV centers form one member of a F¨orster Resonance Energy Transfer (FRET) pair. Due to their broadband emission (> 100 nm), NVs are versatile donors for FRET to systems absorbing in the near infrared spectral range. Highly-promising applications include, e.g., nanoscale imaging of fluorescent molecules or nanomaterials like graphene [2]. Critical parameters for FRET are the NV’s quantum efficiency, charge state stability and NV-sample-distance. Previous experiments used NVs in nanodiamond for FRET [2], however these NVs might suffer from quenching, instability and badly controlled surface termination. We here address this issue by using shallowly implanted NV centers in optimized cylindrical nanostructures [3] used as scanning probes in our homebuilt combination of a confocal and an atomic force microscope. In recent years, two-dimensional materials especially monolayers of semiconducting materials are of major interest in research. Particularly, dichalcogenides like, e.g., tungsten diselenide (WSe2) are promising candidates for a varity of applications [4]. WSe2 emits photons at a wavelength of around 750 nm while absorbing photons below 700 nm [4] which renders WSe2 as a promising FRET partner for NV centers. Here, we present first results towards demonstrating the interaction of NV color centers in single crystal diamond with WSe2. We envisage using quenching of the NV center sued as a donor in FRET in close proximity to the 2D material as a valuable sensing ressource.
关键词: F¨orster Resonance Energy Transfer (FRET),tungsten diselenide (WSe2),nitrogen vacancy (NV) color centers,diamond,two-dimensional materials
更新于2025-09-11 14:15:04