- 标题
- 摘要
- 关键词
- 实验方案
- 产品
-
Collective strong light-matter coupling in hierarchical microcavity-plasmon-exciton systems
摘要： Polaritons are compositional light-matter quasiparticles that arise as a result of strong coupling between the vacuum field of a resonant optical cavity and electronic excitations in quantum emitters. Reaching such a regime is often hard, as it requires materials possessing high oscillator strengths to interact with the relevant optical mode. Two-dimensional transition metal dichalcogenides (TMDCs) have recently emerged as promising candidates for realization of strong coupling regime at room temperature. However, these materials typically provide coupling strengths in the range of 10-40 meV, which may be insufficient for reaching strong coupling with low quality factor resonators. Here, we demonstrate a universal scheme that allows a straightforward realization of strong coupling with 2D materials and beyond. By intermixing plasmonic excitations in nanoparticle arrays with excitons in a WS2 monolayer inside a resonant metallic microcavity, we fabricate a hierarchical system with the collective microcavity-plasmon-exciton Rabi splitting exceeding ~500 meV at room temperature. Photoluminescence measurements of the coupled systems show dominant emission from the lower polariton branch, indicating the participation of excitons in the coupling process. Strong coupling has been recently suggested to affect numerous optical- and material-related properties including chemical reactivity, exciton transport and optical nonlinearities. With the universal scheme presented here, strong coupling across a wide spectral range is within easy reach and therefore exploring these exciting phenomena can be further pursued in a much broader class of materials.
关键词： TMDC,Strong plasmon-exciton coupling,collective Rabi splitting,monolayer WS2
更新于2025-09-23 15:21:21
-
Spatio-temporal coherence in vertically emitting GaAs-based electrically driven polariton lasers
摘要： We report on the implementation of a GaAs-based, vertically emitting electrically pumped polariton laser operated at cryogenic temperatures. The structure consists of a high quality factor AlGaAs/AlAs microcavity (Q ? 15 000) with two stacks of four GaAs quantum wells and features a Rabi splitting of 11 meV. Polariton lasing manifests by a clear threshold in the input–output characteristics of our device with a sharp drop in the emission linewidth and a continuous blueshift of 0.7 meV above threshold with increasing injection current. We measure spatial and temporal coherence of our device in the condensed phase by utilizing interference spectroscopy. Our results clearly demonstrate that electrically driven polariton lasers have promise as monolithic polaritonic sources of coherent light.
关键词： electrically pumped polariton laser,Rabi splitting,coherence,GaAs-based,microcavity
更新于2025-09-23 15:21:01
-
Strong exciton-photon coupling in organic microcavity electroluminescence devices with thiophene/phenylene co-oligomer derivatives
摘要： Organic electroluminescence (EL) devices with surface-emitting microcavity structure were fabricated using vapor-deposited films of thiophene/phenylene co-oligomer derivatives, aiming at polariton formation under electrical excitation. Owing to strong coupling between excitons and photons in the device, we demonstrated the formation of cavity polaritons with a large Rabi-splitting energy (2?Ω = 250 meV). Furthermore, efficient relaxation into the bottom of lower polariton branch was confirmed from angle-resolved EL spectra. In excitation-density dependence, the luminance of microcavity EL devices showed a superlinear increase with an elevation of current density indicating a contribution of triplet excitons.
关键词： polariton,exciton-photon coupling,organic electroluminescence,microcavity,Rabi-splitting
更新于2025-09-19 17:13:59
-
Nonlinear polaritons in a monolayer semiconductor coupled to optical bound states in the continuum
摘要： Optical bound states in the continuum (BICs) provide a way to engineer very narrow resonances in photonic crystals. The extended interaction time in these systems is particularly promising for the enhancement of nonlinear optical processes and the development of the next generation of active optical devices. However, the achievable interaction strength is limited by the purely photonic character of optical BICs. Here, we mix the optical BIC in a photonic crystal slab with excitons in the atomically thin semiconductor MoSe2 to form nonlinear exciton-polaritons with a Rabi splitting of 27 meV, exhibiting large interaction-induced spectral blueshifts. The asymptotic BIC-like suppression of polariton radiation into the far field toward the BIC wavevector, in combination with effective reduction of the excitonic disorder through motional narrowing, results in small polariton linewidths below 3 meV. Together with a strongly wavevector-dependent Q-factor, this provides for the enhancement and control of polariton–polariton interactions and the resulting nonlinear optical effects, paving the way toward tuneable BIC-based polaritonic devices for sensing, lasing, and nonlinear optics.
关键词： nonlinear exciton-polaritons,MoSe2,Rabi splitting,photonic crystal slab,Optical bound states in the continuum
更新于2025-09-19 17:13:59
-
Colloidal Assembly of Aua??Quantum Dota??Au Sandwiched Nanostructures with Strong Plasmona??Exciton Coupling
摘要： Strong plasmon-exciton coupling could occur in hybrid metal-dye/semiconductor nanostructures, where the fast energy exchange between plasmons and excitons leads to two new eigenmodes of the system, known as Rabi splitting. In experiment, strongly coupled nanosystems are difficult to obtain because they require some strict conditions, such as low plasmonic damping, small plasmon mode volume, and good spectral overlap. This work demonstrates strongly coupled metal-semiconductor nanostructures can be constructed using colloidal assembly. Specifically, sandwiched Au-QD-Au nanostructures were created through the assembly of Au nanoparticles and colloidal quantum dots (QDs). The sizes of the QDs and the assembly conditions were varied to control the mode volume of the plasmonic cavity formed between the two Au nanoparticles. With decreased gap size, Rabi splitting was observed in both dark-field scattering and fluorescence spectra of single Au-QD-Au nanostructures. Theoretical simulations revealed that the strong coupling occurred between the excitons and the octupolar plasmon modes.
关键词： Au-QD-Au nanostructures,Rabi splitting,octupolar plasmon modes,plasmon-exciton coupling,colloidal assembly
更新于2025-09-19 17:13:59
-
[IEEE 2019 International Conference on Optical MEMS and Nanophotonics (OMN) - Daejeon, Korea (South) (2019.7.28-2019.8.1)] 2019 International Conference on Optical MEMS and Nanophotonics (OMN) - Hybrid Dielectric Metasurfaces: From Strong Light-Matter Interaction to Extreme Nonlinearities
摘要： We experimentally demonstrate strong coupling between Mie modes of dielectric resonators in a metasurface and intersubband transitions in semiconductor quantum wells that are embedded inside the resonator. The ability to achieve such light-matter coupling creates the possibility to realize ultrathin nonlinear optical devices that are free from complex phase matching requirements and have very high nonlinear conversion efficiencies.
关键词： Rabi splitting,Intersubband transitions,Nonlinear optics,Semiconductor heterostructures,Metasurface
更新于2025-09-16 10:30:52
-
Ultrafast Response of a Hybrid Device Based on Strongly Coupled Monolayer WS <sub/>2</sub> and Photonic Crystals: The Effect of Photoinduced Coulombic Screening
摘要： Quantum interactions between transition metal dichalcogenides (TMDs) and optical cavities are rapidly becoming an appealing research topic since these interactions underly a broad spectrum of optical phenomena. Here, we fabricate a simple device in which coherent strong coupling interactions occur between a photonic crystal (PhC) slab and monolayer tungsten disulfide (WS2). Both steady-state angle-resolved spectroscopy and transient absorption microscopy (TAM) are employed to explore the coupling behavior of this device. Specifically, anticrossing dispersions are observed in the hybrid device, indicating a Rabi splitting of 40.2 meV. A newly formed spectral feature emerges in the transient absorption (TA) spectrum of this polariton device under near-resonant excitation, which is subsequently evidenced to be a signature of the upper hybrid exciton–polariton state. Moreover, by carefully analyzing the ultrafast responses of both bare WS2 and the WS2-PhC polariton device excited both off resonance and near resonance, it is found that nonequilibrium thermal decay induces Coulombic screening in the monolayer WS2, which has a major impact on the formation of exciton–polariton. The results of this work could not only improve the current understanding of photophysics in the strong light–matter coupling regime but also lay the foundation for tailoring the development of TMD-based coherent devices.
关键词： strong coupling,transition metal dichalcogenides,photonic crystals,Rabi splitting,transient absorption microscopy,Coulombic screening
更新于2025-09-16 10:30:52
-
[IEEE 2019 44th International Conference on Infrared, Millimeter, and Terahertz Waves (IRMMW-THz) - Paris, France (2019.9.1-2019.9.6)] 2019 44th International Conference on Infrared, Millimeter, and Terahertz Waves (IRMMW-THz) - Ultrastrong coupling of plasmonic metamaterials and photons in a terahertz photonic crystal cavity
摘要： Light-matter interaction in the strong coupling regime is of profound interest for fundamental quantum optics and applications. Here, we report a new type of strong light-matter interaction of metamaterial ‘quasi-particles’ with photons in a photonic crystal cavity in the terahertz frequency range. The measured Rabi splitting shows a square-root dependence on the density of metamaterial unit cells, even for unit cells from two spatially separated planar metamaterials, indicating nonlocal collective strong interactions. These findings are of interest for the investigation of fundamental strong-coupling phenomena, but also for applications such as ultra-low-threshold terahertz polariton lasing, voltage-controlled modulators and frequency filters, and ultra-sensitive chemical and biological sensing.
关键词： strong coupling,light-matter interaction,metamaterial,nonlocal collective strong interactions,terahertz,Rabi splitting,photonic crystal cavity
更新于2025-09-12 10:27:22
-
Double Rabi Splitting in a Strongly Coupled System of Core-Shell Au@Ag Nanorods and J-Aggregates of Multiple Fluorophores
摘要： The interaction of several components in the strong coupling regime yielding multiple Rabi splittings opens up remarkable possibilities for studies of multimode hybridization and energy transfer, which is of considerable interest in both fundamental and applied science. Here we demonstrate that three different components such as core-shell Au@Ag nanorods and J-aggregates of two different dyes, can be integrated into a single hybrid structure, which leads to strong collective exciton-plasmon coupling and double-mode Rabi splitting totaling 338 meV. We demonstrate strong coupling in these multicomponent plexitonic nanostructures by means of magnetic circular dichroism spectroscopy, and demonstrate strong magneto-optical activity for the three hybridized states resulting from this coupling. The J-aggregates of two different non-magnetic dyes interact with metal nanoparticles effectively, achieving magnetic properties due to the hybridization of electronic excitations in the three-component system.
关键词： magnetic circular dichroism,double Rabi splitting,J-aggregates,plexciton,Strong coupling,magneto-optical activity
更新于2025-09-12 10:27:22
-
Strong Coupling in Microcavity Structures: Principle, Design, and Practical Application
摘要： When interaction between light and matter is in the strong coupling region, matter has a significant influence on the whole system, with potential to develop low-power active optical devices. Strong coupling can verify some basic problems of quantum physics, and it is an ideal system to study light–matter interaction, providing an intuitive and accurate demonstration of some pure quantum effects with small mass and easy optical control. Here, the most important advances in strong coupling in recent years are described. Of late, an extensive series of experimental and theoretical findings, and remarkable achievements have been made in this field. Strong coupling between cavities and some new materials such as semiconductors, two-dimensional (2D) material, and quantum dots (QDs) are the focus of research in this field. Another field that has made outstanding progress is the application of this optical phenomenon, including resonance-enhanced Raman and infrared spectra, nanolasers, and cavity-enhanced sensing. Furthermore, the potential in this field arises for future quantum information and quantum optical devices. It is now developing at a very fast rate and can be predicted to have broad prospects for development in the future. Some prospects in terms of design and application are included.
关键词： strong coupling,vacuum Rabi splitting,optical devices,quantum optics
更新于2025-09-10 09:29:36