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Discrimination of entangled photon pair from classical photons by de Broglie wavelength
摘要： Quantum optics largely relies on the fundamental concept that the diffraction and interference patterns of a multi-partite state are determined by its de Broglie wavelength. in this paper we show that this is still true for a mixed state with one sub-system being in a classical coherent state and one being in entangled state. We demonstrate the quantum-classical light discrimination using de Broglie wavelength for the states with all classical parameters being the same.
关键词： entangled photons,de Broglie wavelength,quantum optics,classical photons,quantum-classical discrimination
更新于2025-09-23 15:21:01
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Continuous-wave dual-wavelength operation of the in-band diode-pumped Nd:GdVO4/Nd:YVO4 composite laser with controllable spectral power ratio
摘要： Controllable continuous-wave dual-wavelength laser operation of a Nd:GdVO4/Nd:YVO4 composite crystal at 1063 and 1064 nm was demonstrated using in-band diode pumping around 912 nm. The spectral power ratio of the two laser wavelengths could be adjusted simply by controlling the pump wavelength of the laser diode via temperature. The laser produced the maximum total output power of 4.48 W. The maximum slope and optical-to-optical efficiency with respect to the absorbed pump power were 43.8% and 38.8%, respectively.
关键词： in-band diode pumping,Nd:GdVO4/Nd:YVO4 composite crystal,dual-wavelength laser,spectral power ratio,continuous-wave operation
更新于2025-09-23 15:21:01
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Robust Wavelength-Converting and Lasing Media from Wafer-Scale Inorganic Perovskites Enabled by a Protective Surface Layer
摘要： Despite that the inorganic halide perovskites show great promise in wavelength-conversion and lasing applications, the stability and scalability remain as the obstruction toward practical applications. Herein, we, for the first time, employ the wafer-scale inorganic perovskite single crystals to address the above issue. Our spectroscopic analysis reveals that the carrier trapping on the crystal surface is the most probable culprit to hinder the optical amplification for the weak-penetrating one-photon pumping, whilst, the interior of the crystal preserves intact and show low-threshold stimulated emission by two-photon absorption in the near infrared regime. Thanks to the effective protection from the surface layer, the stimulated emission maintains 90% of the initial intensity upon uninterrupted pumping of 4 hours and shows nearly constant threshold upon long-term storage without any encapsulation (> one year). By exploiting a parallel-mirror cavity, an optically pumped wavelength-converting and laser device featuring a spatially coherent output beam is constructed. Our finding greatly advances the development of practical coherent light sources based on halide perovskites.
关键词： wavelength-conversion,lasing,scalability,two-photon absorption,inorganic halide perovskites,stability,coherent light sources,stimulated emission
更新于2025-09-23 15:21:01
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Interaction effect of LED color temperatures and light-protective additive packaging on photo-oxidation in milk displayed in retail dairy case
摘要： Effect of varied LED color temperatures on photo-oxidation in 2 % fat milk and protection efficiency of packaging with and without light-protective additives (LPA) under different color temperatures was firstly evaluated. Riboflavin (Rb) is one of the critical photo-sensitizers in 2 % milk when exposed to LED light. Higher color temperature with higher relative intensity of Rb absorbance region resulted in lower Rb and vitamin A retention, lower dissolved oxygen content, and higher TBARS value in milk packaged with non-LPA packaging. Yellow pigmented packaging that completely blocked the Rb absorbance region of all three LED color temperatures successfully reduced the rate of degradation of milk nutrients and flavor. TiO2-added packaging partially block the destructive light wavelength; higher level of TiO2 provided a longer protection on milk freshness. Combination of appropriate LED color temperature and LPA-packaging provided a cost-effective solution for minimizing photo-oxidation in retail dairy case.
关键词： color temperature,oxidation,freshness,milk,packaging,light wavelength,LED
更新于2025-09-23 15:21:01
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Exploiting Wavelength Orthogonality for Successive Photoinduced Polymerization-Induced Self-Assembly and Photo-Crosslinking
摘要： We report a facile benchtop process for the synthesis of cross-linked polymeric nanoparticles by exploiting wavelength-selective photochemistry to perform orthogonal photoinduced polymerization-induced self-assembly (Photo-PISA) and photo-crosslinking processes. We first established that the water-soluble photocatalyst, zinc meso-tetra(N-methyl-4-pyridyl) porphine tetrachloride (ZnTMPyP) could activate the aqueous PET-RAFT dispersion polymerization of hydroxypropyl methacrylate (HPMA). This photo-PISA process could be conducted under low energy red light (λ max = 595 nm, 10.2 mW/cm2) and without deoxygenation due to the action of the singlet oxygen quencher, biotin (vitamin B7), which allowed for the synthesis of a range of nanoparticle morphologies (spheres, worms, and vesicles) directly in 96-well plates. To perform wavelength selective nanoparticle cross-linking, we added the photoresponsive monomer, 7-[4-(trifluoromethyl)coumarin] methacrylamide (TCMAm) as a comonomer without inhibiting the evolution of the nanoparticle morphology. Importantly, under red light, exclusive activation of the photo-PISA process occurs, with no evidence of TCMAm dimerization under these conditions. Subsequent switching to a UV source (λ max = 365 nm, 10.2 mW/cm2) resulted in rapid cross-linking of the polymer chains, allowing for retention of the nanoparticle morphology in organic solvents. This facile synthesis of cross-linked spheres, worms, and vesicles demonstrates the utility of orthogonal light-mediated chemistry for performing decoupled wavelength selective chemical processes.
关键词： photoinduced polymerization-induced self-assembly,wavelength orthogonality,polymeric nanoparticles,photo-crosslinking,PET-RAFT polymerization
更新于2025-09-23 15:21:01
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Near-infrared nanosecond-pulsed laser-activated high efficient intracellular delivery mediated by nano-corrugated mushroom-shaped gold-coated polystyrene nanoparticles
摘要： Here, efficient intracellular delivery of molecules with high cell viability is reported using nanosecond-pulsed laser-activated plasmonic photoporation mediated by high-aspect-ratio nano-corrugated mushroom-shaped gold-coated polystyrene nanoparticles (nm-AuPNPs) at near-infrared wavelength. Upon laser illumination, nm-AuPNPs exhibit greater plasmonic extinction than spherical AuPNPs, which increase their energy efficiency and reduce the necessary illumination of light, effectively controlling cell damage and improving delivery efficiency. Nm-AuPNPs exhibit surface plasmon absorption at near infrared region with peak at 945 nm. Pulsed laser illumination at this plasmon peak triggers explosive nanobubbles, which create transient membrane pores, allowing the delivery of dyes, quantum dots and plasmids into the cells. The results can be tuned by laser fluence, exposure time, molecular size and concentration of nm-AuPNPs. The best results are found for CL1-0 cells, which yielded a 94% intracellular PI dye uptake and ~100% cell viability at 35 mJ/cm2 laser fluence for 945 nm wavelength. Thus, the presented approach has proven to have an inevitable potential for biological cell research and therapeutic applications.
关键词： near-infrared wavelength,intracellular delivery,nanosecond-pulsed laser,gold-coated polystyrene nanoparticles,plasmonic photoporation
更新于2025-09-23 15:21:01
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Temperature and Emissivity Inversion Accuracy of Spectral Parameter Changes and Noise of Hyperspectral Thermal Infrared Imaging Spectrometers
摘要： The emergence of hyperspectral thermal infrared imaging spectrometers makes it possible to retrieve both the land surface temperature (LST) and the land surface emissivity (LSE) simultaneously. However, few articles focus on the problem of how the instrument?s spectral parameters and instrument noise level affect the LST and LSE inversion errors. In terms of instrument development, this article simulated three groups of hyperspectral thermal infrared data with three common spectral parameters and each group of data includes tens of millions of simulated radiances of 1525 emissivity curves with 17 center wavelength shift ratios, 6 full width at half maximum (FWHM) change ratios and 6 noise equivalent differential temperatures (NEDTs) under 15 atmospheric conditions with 6 object temperatures, inverted them by two temperature and emissivity separation methods (ISSTES and ARTEMISS), and analyzed quantitatively the effects of the spectral parameters change and noise of an instrument on the LST and LSE inversion errors. The results show that: (1) center wavelength shifts and noise affect the inversion errors strongly, while FWHM changes affect them weakly; (2) the LST and LSE inversion errors increase with the center wavelength shift ratio in a quadratic function and increase with FWHM change ratio slowly and linearly for both the inversion methods, however they increase with NEDT in an S‐curve for ISSTES while they increase with NEDT slightly and linearly for ARTEMISS. During the design and development of a hyperspectral thermal infrared instrument, it is highly recommended to keep the potential center wavelength shift within 1 band and keep NEDT within 0.1K (corresponding LST error < 1K and LSE error < 0.015) for normal applications and within 0.03K (corresponding LST error < 0.5K and LSE error < 0.01) for better application effect and level.
关键词： inversion error,hyperspectral thermal infrared,FWHM change,instrument noise,center wavelength shift,temperature and emissivity separation
更新于2025-09-23 15:21:01
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Multi-wavelength colloidal quantum dot lasers in distributed feedback cavities
摘要： Lasers with multi-wavelength colloidal quantum dots (CQDs) can be achieved using complex grating structures and ?exible substrate. The structure contains graduated periods and rectangular cavity fabricated through interference lithography, which acts as the distributed feedback cavity. A layer of densely packed CQD ?lm is deposited on the cavity via spin coating technique. The performance of CQD lasers based on di?erent distributed feedback cavities is investigated. Multi-wavelength lasing is achieved based on a ?exible rectangular cavity.
关键词： ?exible,tunable,distributed feedback,quantum dots lasers,multi-wavelength
更新于2025-09-23 15:21:01
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Organic Printed Core-Shell Heterostructure Arrays: A Universal Approach to All-Color Laser Display Panels
摘要： We demonstrate a universal approach for realizing dual-wavelength lasing in organic core-shell structured microlaser arrays, which show great promise in serving as all-color laser display panels. By alternately printing hydrophilic and hydrophobic laser dye solutions on preprocessed substrates, we successfully obtained precisely patterned core-shell heterostructure arrays. The spatially-separated core and shell independently function as optical resonators to support dual-wavelength tunable microlasers in each heterostructure. Such a general method enables to flexibly control the lasing wavelength of the core-shell microlasers across a wide spectral range by systematically designing the gain media. Using as-prepared microlaser arrays as display panels, we achieved full-color laser displays, representing an achievable color gamut much larger than that of standard RGB space. These results may provide new insights for design concepts and device construction for novel optoelectronic applications.
关键词： organic heterostructure,laser display,dual-wavelength laser,core-shell structure,laser array
更新于2025-09-23 15:21:01
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Optimizing the performance of ZnO/Au/MgZnO/SiO2 sandwich structured UV photodetectors by surface plasmons in Ag nanoparticles
摘要： The dual-wavelength UV photodetector (PD) with sandwich structure of ZnO/Au/MgZnO/SiO2 was fabricated and investigated with an emphasis on the effects of the Ag nanoparticles localized surface plasmons (LSPs). The results demonstrated that the modification in Ag nanoparticle (NP) position played a remarkable influence on the performance of dual-wavelength UV photodetectors. In comparison with decorating Ag NPs on the surface of the PDs, embedding Ag NPs between the MgZnO and ZnO films could improve two peak responsivities (caused by MgZnO and ZnO layers) significantly. By calculating the responsivities enhancement ratio of double layers (MgZnO and ZnO), the results indicated that the enhancement ratio of MgZnO is higher than that of ZnO. This was ascribed to LSPs of energy match with MgZnO which was superior to ZnO. This work described a creative method for increasing the performance of dual-wavelength UV PDs.
关键词： MgZnO,Ag nanoparticles,Dual wavelength,ZnO,Surface plasmons,UV photodetectors
更新于2025-09-23 15:21:01