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Morphology Effect of 1D ZnO Nanostructures Designed by Hydrothermal and Thermal Annealing for Fast Ultraviolet Photodetector Applications
摘要： Zinc oxide (ZnO) nanorods were grown on a ZnO seed layer using the hydrothermal method and subsequently annealed at temperatures of 400–800 °C. The ZnO nanorods annealed at 400 °C exhibited morphology similar to that of the unannealed ZnO nanorods. However, the tips of the ZnO nanorods gradually became rounded and their density and diameter increased with an increase in the annealing temperature. The intensity of the near-band-edge emission increased gradually with an increase in the annealing temperature from 400 to 600 °C but decreased sharply in the case of the nanorods annealed at 800 °C. With respect to the deep-level emissions, broad yellow, orange, and green emissions were observed. Further, the low-temperature photoluminescence spectrum measured at 12 K of the ZnO nanorods annealed at 600 °C contained a donor-bound exciton emission, as well as emissions related to the donor-acceptor pair transition and the first-order and second-order longitudinal optical phonon replicas of the donor-acceptor pair transition. Finally, with respect to the photoresponse, the dark current and photocurrent of the nanorods decreased and their photosensitivity increased with the increase in the annealing temperature.
关键词： Ultraviolet photodetector,Zinc oxide,Photosensitivity,Photoluminescence,Hydrothermal method
更新于2025-09-23 15:19:57
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Design of a Surface Plasmon Resonance-Enhanced ZnO Ultraviolet Photodetector Based on a Sub-wavelength Metal Grating Covered with a High-Refractive-Index Medium
摘要： To realize a surface plasmon resonance-enhanced zinc oxide (ZnO) ultraviolet photodetector based on a sub-wavelength metal grating, we take advantage of the sensitivity of the resonance condition of a sub-wavelength metal grating to the refractive index of the surrounding medium. We theoretically design a sub-wavelength Ag grating covered with a high-refractive-index medium layer and apply it to a ZnO ultraviolet photodetector. By optimizing the parameters (angle of incidence, grating period, grating spacing, grating thickness, high-refractive-index medium layer thickness, refractive index of the covering), the optical ?eld is localized at the interface of the sub-wavelength Ag grating and the ZnO thin ?lm; that is, surface plasmon resonance is realized within the device. Compared with the device without a high-refractive-index medium layer, the maximum absorption enhancement factor of the designed device can reach up to 108. This work will provide theoretical guidance to realize a surface plasmon resonance-enhanced ZnO ultraviolet photodetector with a sub-wavelength metal grating.
关键词： ultraviolet photodetector,ZnO,sub-wavelength metal grating,Surface plasmon resonance
更新于2025-09-23 15:19:57
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High Responsivity and High Rejection Ratio Self-Powered Solar-Blind Ultraviolet Photodetector Based on PEDOT:PSS/β-Ga2O3 Organic/Inorganic p-n Junction
摘要： A high responsivity self-powered solar-blind deep UV (DUV) photodetector with high rejection ratio was proposed based on inorganic/organic hybrid p-n junction. Owing to the high crystalized β-Ga2O3 and excellent transparent conductive polymer PEDOT:PSS, the device exhibited ultrahigh responsivity of 2.6 A/W at 245 nm with a sharp cut off wavelength at 255 nm without any power supply. The responsivity is much larger than that of previous solar-blind DUV photodetectors. Moreover, the device exhibited an ultrahigh solar-blind/UV rejection ratio (R245 nm /R280 nm) of 103, which is two orders of magnitude larger than the average value ever reported in Ga2O3-based solar-blind photodetectors. In addition, the photodetector shows a narrow band-pass response of only 17 nm in width. This work might be of great value in developing high wavelength selective DUV photodetector with respect to low cost for future energy-efficient photoelectric devices.
关键词： Self-Powered,PEDOT:PSS/β-Ga2O3,Plasmonics and Optoelectronics,Organic/Inorganic p-n Junction,Energy Conversion and Storage,High Rejection Ratio,High Responsivity,Solar-Blind Ultraviolet Photodetector
更新于2025-09-19 17:13:59
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[IEEE 2018 IEEE 8th International Conference Nanomaterials: Application & Properties (NAP) - Zatoka, Ukraine (2018.9.9-2018.9.14)] 2018 IEEE 8th International Conference Nanomaterials: Application & Properties (NAP) - Semi-transparent UV Photodetectors Based on the Nanostructured n-ZnO/p-CuI and n-ZnO/p-NiO Diode Heterojunctions Prepared by Low Temperature Solution Growth
摘要： In this work we investigate wide band-gap bipolar diode nanostructured heterojunctions prepared by low temperature solution growth. The crystal structure and optical properties of the pulsed electrodeposited zinc oxide nanorod arrays and nickel oxide and copper iodide films grown via Successive Ionic Layer Adsorption and Reaction (SILAR) technique, and also diode parameters and photoelectric characteristics of the heterojunctions show that they are promising for a fabrication of low cost and portable semi-transparent photodetectors of soft ultraviolet light.
关键词： ultraviolet photodetector,copper iodide,nickel oxide,nanocrystal structure,specific detectivity,zinc oxide
更新于2025-09-16 10:30:52
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Enhanced photoresponse in ZnO nanorod array/p-GaN self-powered ultraviolet photodetectors via coupling with CuO nanostructures
摘要： ZnO nanorod arrays (ZnO NRAs) coupled with coral-like CuO nanostructures (CuO CLNs) were prepared by low-temperature hydrothermal method. Self-powered ultraviolet (UV) photodetectors (PDs) based on ZnO NRAs/CuO CLNs/p-GaN heterostructure were fabricated via a direct-contact method. Under UV illumination (1.46 mW cm?2), the ratios of photocurrent to dark current (Iphoto/Idark), photo-responsivity and speci?c detectivity for the ZnO NRAs/CuO CLNs/p-GaN heterojunction self-powered PD were estimated to be 1143, 1.44 mA W?1 and 5.9×1010 cm Hz1/2/W at 0 V, which were about ～187, ～104 and ～153 times greater than those of the ZnO NRAs/p-GaN self-powered PD, respectively. Moreover, the PD displayed faster response time, excellent stability and repeatability by coupling with CuO CLNs. The mechanism of the enhanced photoresponse performance was discussed through the energy band diagram.
关键词： self-powered,CuO nanostructures,ultraviolet photodetector,ZnO nanorods
更新于2025-09-16 10:30:52
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[IEEE 2019 20th International Conference on Solid-State Sensors, Actuators and Microsystems & Eurosensors XXXIII (TRANSDUCERS & EUROSENSORS XXXIII) - Berlin, Germany (2019.6.23-2019.6.27)] 2019 20th International Conference on Solid-State Sensors, Actuators and Microsystems & Eurosensors XXXIII (TRANSDUCERS & EUROSENSORS XXXIII) - A High-Performance Self-Powered UV Photodetector Based on Self-Doping TIO <sub/>2</sub> Nanotube Arrays
摘要： In this paper, we present a high-performance self-powered ultraviolet (UV) photodetector using electrochemical micro-porous-channel arrays based on a cost-effective and environment-friendly black TiO2 nanotube arrays (BTNAs) and polysulfide (S2-/Sx2-) electrolyte. By self-doping TiO2 the concentration and lifetime of UV photo-generated carriers are increased due to increasing oxygen vacancies and Ti3+ defects in BTNAs, effectively enhancing the carrier transport and multiple exciton effect of carriers, and thus the self-powered UV photodetector based on electrochemical micro-porous-channel arrays demonstrates a high photoresponsivity of ~22 mA/W and high-speed photoresponse of ~4 ms in rise and decay time.
关键词： TiO2 nanotube arrays,self-powered sensors,electrochemical sensors,ultraviolet photodetector
更新于2025-09-16 10:30:52
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Nanoplasmonic 1D Diamond UV Photodetectors with High Performance
摘要： Diamond nanowires have recently drawn substantial attention due to their unique physical and chemical properties for electrochemical sensors, optoelectronics, and nanophotonics applications. However, diamond nanowire based ultraviolet photodetectors have not been reported because of the challenges involved in synthesizing crystalline diamond nanowires with controllable morphologies and, more fundamentally, the material’s high carrier concentration with low mobilities that limits the obtainable photoresponsivity. The synergetic integration of ultrananocrystalline diamond (UNCD) nanowires with nanoplasmonic enhancement by noble metal nanoparticles is a very promising approach to overcome these shortcomings. Here we report the fabrication of boron doped ultrananocrystalline diamond nanowires functionalized with the platinum nanoparticles to form self-powered ultraviolet photodetectors that exhibit an ultrahigh photoresponsivity of 388 Amp/Watt at 300 nm wavelength, a fast response time around 20 ms, and a good UV/visible rejection ratio of about five orders of magnitude under zero-bias condition.
关键词： ultraviolet photodetector,nanowire,metal nanoparticle,ultrananocrystalline diamond,nanoplasmonics
更新于2025-09-12 10:27:22
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Catalyst-Free Growth of a Zn2GeO4 Nanowire Network for High-Performance Transfer-Free Solar-Blind Deep UV Detection
摘要： Solar-blind deep-ultraviolet (DUV) photodetectors have attracted wide attention because of their extensive military and civil applications. The ternary oxide Zn2GeO4 is an ideal material with a wide bandgap (Eg = 4.69 eV). In this work, DUV photodetectors based on a ternary Zn2GeO4 nanowire (NW) network were fabricated on SiO2/Si substrates. Reactive ion etching of the SiO2/Si wafer was used to grow the NW network to avoid contamination of the Au catalyst during synthesis of the Zn2GeO4 NW network via high-temperature chemical vapor deposition. Photodetectors based the Zn2GeO4 NW revealed fast response and recovery times, which is attributed to the unique cross-junction barrier-dominated conductance of the NW network. Results showed that the ternary oxide-based NW network is an ideal building block for nanoscale solar-blind photodetectors with superior performance.
关键词： Zn2GeO4 nanowire,ultraviolet photodetector,catalyst-free
更新于2025-09-10 09:29:36
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Comprehensive Pyro‐Phototronic Effect Enhanced Ultraviolet Detector with ZnO/Ag Schottky Junction
摘要： As a coupling effect of pyroelectric and photoelectric effect, pyro-phototronic effect has demonstrated an excellent tuning role for fast response p–n junction photodetectors (PDs). Here, a comprehensive pyro-phototronic effect is utilized to design and fabricate a self-powered and flexible ultraviolet PD based on the ZnO/Ag Schottky junction. By using the primary pyroelectric effect, the maximal transient photoresponsivity of the self-powered PDs can reach up to 1.25 mA W?1 for 325 nm illumination, which is improved by 1465% relative to that obtained from the steady-state signal. The relative persistent secondary pyroelectric effect weakens the height of Schottky barrier, leading to a reduction of the steady-state photocurrent with an increase in the power density. When the power density is large enough, the steady-state photocurrent turns into a reverse direction. The corresponding tuning mechanisms of the comprehensive pyro-phototronic effect on transient and steady-state photocurrent are revealed based on the bandgap diagrams. The results may help us to further clarify the mechanism of the pyro-phototronic effect on the photocurrent and also provide a potential way to optimize the performance of self-powered PDs.
关键词： ultraviolet photodetector,Schottky junction,secondary pyroelectric effect,pyro-phototronic effect,self-powered
更新于2025-09-04 15:30:14