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Nanomechanical Microfluidic Mixing and Rapid Labelling of Silica Nanoparticles with Allenamide to Thiol Covalent Link for Bioimaging
摘要： Rapid surface functionalization of nanomaterials using covalent linkage following ‘green chemistry’ remains challenging and the quest for developing simple protocols are persisting. We report a nanomechanical microfluidic approach for the coupling of allenamide functionalized organic derivatives on the surface of thiol modified silica nanoparticles using allenamide-thiol chemistry. The coupling principle involves the use of a microfluidic surface acoustic wave (SAW) device that generates acoustic streaming based chaotic fluid micromixing that enables mixing of laterally flowing fluids containing active components. This approach was used to demonstrate the direct surface labeling of thiol modified silica nanoparticles using a selected group of modified fluorescence tags containing allenamide handles and achieved a total efficiency of 83-90 %. This green approach enabled a highly efficient surface functionalization in aqueous conditions, with tunable control over the conjugation process via the applied field. The dye labelled silica particles were characterized using various analytical techniques and found to be biocompatible with a potential in live cell bioimaging. It is envisaged that this bioconjugation strategy will find numerous applications in the field of bioimaging and drug delivery.
关键词： microfluidics,surface acoustic wave (SAW),allenamide-thiol chemistry,bioimaging,nanoparticles
更新于2025-09-23 15:23:52
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Behavior of Al/Cu/Ti electrodes in surface acoustic wave filter at high power
摘要： Driven by the need for high data-rates and continuous reduction in device size, surface acoustic wave filters are required to work under increasingly high power. In this work, a series of 2.7 GHz surface acoustic wave filters with Al/Cu/Ti three-layered electrode were fabricated and loaded with high power. Those three-layered electrodes showed weaker texture but higher stability than Al-Cu alloy electrode at high power. Morphologies, microstructures and elements distribution in cross section of fingers were analyzed carefully before and after high power loading. Results show that the circular-arc-shaped outline of fingers were appeared in most samples after high power loading, and the number of gains in the finger cross section changed from some into several with much larger volume. The features of distribution of Cu atoms also coincided with these microstructures. By finite element method and phase diagram analysis, the higher stability of Al/Cu/Ti three-layered electrodes are attributed to precipitation of θ-CuAl2 in the bottom edge of electrode finger and Cu-doped α-Al in the center top.
关键词： stress,Al-Cu alloy,high power,surface acoustic wave filter,three-layered electrode
更新于2025-09-23 15:23:52
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Surface Acoustic Wave Gyroscopic Effect in an Interdigital Transducer
摘要： The surface acoustic wave (SAW) gyroscopic effect in an interdigital transducer (IDT) deposited on a piezoelectric substrate is different from that in the piezoelectric substrate due to a reflection induced by IDT. In this work, an extended coupling-of-mode (COM) model including the gyroscopic effect and the reflection was developed to analyze the SAW gyroscopic effect. First, dispersion characteristics parameters of SAW were fitted according to the data derived using the finite element method (FEM). Then, variations of stop band edge frequency were calculated using the extended COM theory by integrating dispersion characteristics parameters into the COM model. We compared its results with those obtained via FEM analysis to confirm the proposed model's validity. We found that the variation in stop band edge frequency related to gyroscope effect reached the maximum value with a zero reflectivity value. For split IDT, the sensitivity of gyroscope effect is 0.036 Hz/rad/s with a lower than 1% normalized thickness. Conversely, the value of sensitivity was almost zero for bidirectional IDT and electrode width controlled single-phase unidirectional transducer (EWC/SPUDT).
关键词： interdigital transducer,surface acoustic wave,gyroscopic effect
更新于2025-09-23 15:23:52
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Monitoring of Film Qualities of Amorphous SiO2 films/Si(100) Substrates by Measuring Bulk and Surface Acoustic Waves in Terms of Brillouin Spectroscopy
摘要： Acoustic properties of amorphous SiO2 thin films deposited on the Si(100) substrate were investigated by using Brillouin spectroscopy. The Brillouin spectrum was obtained by tilting the sample to investigate both the longitudinal acoustic (LA) mode and the surface acoustic wave (SAW) modes. Sound velocities of both modes, the two elastic moduli (longitudinal and shear moduli), and the Poisson ratio of the film could be obtained by combining the Brillouin data and the measured refractive index. The longitudinal sound velocity and the longitudinal elastic modulus increased with increasing Ar ratio in the Ar:O2 gas mixture, which was attributed to the better stoichiometry of the film grown at higher Ar ratio.
关键词： Brillouin scattering,Surface acoustic wave,SiO2 film
更新于2025-09-23 15:22:29
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Anisotropy of acoustic and thermal expansion properties of TlInSe <sub/>2</sub> crystals
摘要： Based on experimental studies of acoustic wave velocities in TlInSe2 crystals, all components of their elastic stiffness and compliance tensors are determined. TlInSe2 has three acoustic axes parallel to the principal crystallographic directions. The lowest velocities of acoustic eigenwaves are used to estimate the acousto-optic figure of merit. We analyse deviations from purely longitudinal and transverse polarization states, as well as the obliquity of acoustic energy flow. Temperature dependences of strains along the three principal crystallographic directions and of acoustic wave velocities v11, v22 and v33 are measured. Anomalous behaviour of these parameters occur at T1≈245 K and T2≈145 K. It is shown that the symmetry of TlInSe2 becomes lower than tetragonal below the temperature point T1.
关键词： TlInSe2 crystals,Ferroics,elastic properties,thermal expansion,anisotropy,acoustic wave velocity
更新于2025-09-23 15:21:21
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[ACM Press the 2017 2nd International Conference - Wuhan, China (2017.11.07-2017.11.09)] Proceedings of the 2017 2nd International Conference on Communication and Information Systems - ICCIS 2017 - Effect of Concentration on Surface Acoustic Wave Velocity in A Rayleigh-type Biosensor
摘要： To predict the propagation velocity of different concentrations of bovine serum albumin (BSA) in a Rayleigh-type biosensor, we derived a new calculation method for a Rayleigh surface acoustic wave (SAW) device. The method can calculate propagation velocities of leaky Rayleigh waves and Rayleigh waves when liquid is placed in the groove of a Rayleigh-type SAW device. Different concentration of BSA proteins were used to evaluate the effect of these concentrations. In this study, we used different concentrations of BSA and a Rayleigh-type SAW device consisted of grooves of 0.25 mm width and 0.26 mm height and grooves of 0.40 mm width and 0.25 mm height, quartz as the substrate and interdigital transducers (IDT) with a 25.00 mm distance. The frequency of the Rayleigh-type SAW device was set to 157.6 MHz. Our data suggests that the propagation velocity of SAWs depends mainly upon BSA protein concentration and the size of groove. At the same concentration of BSA, the propagation acoustic wave velocity of BSA depends on the size of groove. The results showed the 0.40 mm width-0.25 mm height groove was more suitable than the 0.25 mm width-0.26 mm height groove for studying the propagation velocity of wave with liquid in a Rayleigh-type SAW device. With the propagation velocity decreased when the concentration of BSA protein increased.
关键词： Surface acoustic wave (SAW),Rayleigh-type SAW device,Leaky Rayleigh wave,Bovine serum albumin (BSA),Rayleigh wave
更新于2025-09-23 15:21:01
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The influence of acoustic deformation on the recombination radiation in InAs/GaAs heterostructure with InAs quantum dots
摘要： In the framework of electron-deformation model, the influence of deformation on the energy spectrum of electrons and holes in InAs/GaAs heterostructure with InAs quantum dots (QD) is investigated. The influence of acousto-electronic effects on the modulation of radiation energy at the recombination transition between the ground states of electron and hole in InAs/GaAs heterostructure with InAs quantum dots is investigated. The nature of the amplitude dependence of the modulation of the recombination radiation energy on the QD size and the amplitude of the mechanical stress created by the acoustic wave on the surface of the matrix is established.
关键词： Deformation,Modulation of the energy,Acoustic wave,Quantum dot,Energy of electron and hole
更新于2025-09-23 15:21:01
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New approach to detection of guided waves with negative group velocity: Modeling and experiment
摘要： A new method for detecting the forward and backward acoustic waves in the piezoelectric plates by using a system of the acoustically isolated interdigital transducers (IDT) with the different spatial period is developed. This method was tested on the piezoelectric acoustic modes A1 and SH1 propagating in Y-X LiNbO3 plate. Theoretical analysis has shown that the SH1 mode in the entire frequency range represented a forward wave. At that the dispersion dependence of the A1 mode near the cutoff frequency has a smooth transition from a forward wave to a backward one with decreasing frequency. In order to experimentally observe this transition 19 IDTs with different periods were deposited on a single lithium niobate plate. The measurement of the frequency dependence of the real part of the electrical impedance of these IDTs showed that for SH1 mode the resonance frequency decreased monotonically with a growth in the spatial period. This behavior corresponded to a forward wave. For A1 mode the resonance frequency initially decreased with the growth of the IDT period and then began to increase after reaching a value of ZGV frequency. This behavior is explained by the smooth transition from the region of the forward wave to the region of the backward wave. The calculation of the frequency dependences of the real part of the electrical impedance of each transducer for the waves considered, carried out by the finite element method, turned out to be in good agreement with the experiment.
关键词： interdigital transducer,forward and backward plate acoustic wave,phase and group velocities,dispersion dependencies,finite element analysis,electrical impedance
更新于2025-09-23 15:21:01
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Single-photon emission from single-electron transport in a SAW-driven lateral light-emitting diode
摘要： The long-distance quantum transfer between electron-spin qubits in semiconductors is important for realising large-scale quantum computing circuits. Electron-spin to photon-polarisation conversion is a promising technology for achieving free-space or fibre-coupled quantum transfer. In this work, using only regular lithography techniques on a conventional 15 nm GaAs quantum well, we demonstrate acoustically-driven generation of single photons from single electrons, without the need for a self-assembled quantum dot. In this device, a single electron is carried in a potential minimum of a surface acoustic wave (SAW) and is transported to a region of holes to form an exciton. The exciton then decays and creates a single optical photon within 100 ps. This SAW-driven electroluminescence, without optimisation, yields photon antibunching with g(2)(0) = 0.39 ± 0.05 in the single-electron limit (g(2)(0) = 0.63 ± 0.03 in the raw histogram). Our work marks the first step towards electron-to-photon (spin-to-polarisation) qubit conversion for scaleable quantum computing architectures.
关键词： quantum computing,GaAs quantum well,electron-spin qubits,surface acoustic wave,single-photon emission
更新于2025-09-23 15:19:57
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Development of Pd/TiO2 Porous Layers by Pulsed Laser Deposition for Surface Acoustic Wave H2 Gas Sensor
摘要： The influence of sensitive porous films obtained by pulsed laser deposition (PLD) on the response of surface acoustic wave (SAW) sensors on hydrogen at room temperature (RT) was studied. Monolayer films of TiO2 and bilayer films of Pd/TiO2 were deposited on the quartz substrates of SAW sensors. By varying the oxygen and argon pressure in the PLD deposition chamber, different morphologies of the sensitive films were obtained, which were analyzed based on scanning electron microscopy (SEM) images. SAW sensors were realized with different porosity degrees, and these were tested at different hydrogen concentrations. It has been confirmed that the high porosity of the film and the bilayer structure leads to a higher frequency shift and allow the possibility to make tests at lower concentrations. Thus, the best sensor, Pd-1500/TiO2-600, with the deposition pressure of 600 mTorr for TiO2 and 1500 mTorr for Pd, had a frequency shift of 1.8 kHz at 2% hydrogen concentration, a sensitivity of 0.10 Hz/ppm and a limit of detection (LOD) of 1210 ppm. SAW sensors based on such porous films allow the detection of hydrogen but also of other gases at RT, and by PLD method such sensitive porous and nanostructured films can be easily developed.
关键词： bilayer films,pulsed laser deposition (PLD),palladium,hydrogen sensor,surface acoustic wave (SAW),Pd/TiO2,porous morphology,titanium dioxide
更新于2025-09-23 15:19:57