- 标题
- 摘要
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- 实验方案
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Flexible and Selfa??Powered Photodetector Arrays Based on Alla??Inorganic CsPbBr <sub/>3</sub> Quantum Dots
摘要： Flexible devices are garnering substantial interest owing to their potential for wearable and portable applications. Here, flexible and self-powered photodetector arrays based on all-inorganic perovskite quantum dots (QDs) are reported. CsBr/KBr-mediated CsPbBr3 QDs possess improved surface morphology and crystallinity with reduced defect densities, in comparison with the pristine ones. Systematic material characterizations reveal enhanced carrier transport, photoluminescence efficiency, and carrier lifetime of the CsBr/KBr-mediated CsPbBr3 QDs. Flexible photodetector arrays fabricated with an optimum CsBr/KBr treatment demonstrate a high open-circuit voltage of 1.3 V, responsivity of 10.1 A W?1, specific detectivity of 9.35 × 1013 Jones, and on/off ratio up to ≈104. Particularly, such performance is achieved under the self-powered operation mode. Furthermore, outstanding flexibility and electrical stability with negligible degradation after 1600 bending cycles (up to 60°) are demonstrated. More importantly, the flexible detector arrays exhibit uniform photoresponse distribution, which is of much significance for practical imaging systems, and thus promotes the practical deployment of perovskite products.
关键词： self-powered devices,perovskites,flexible devices,photodetector arrays
更新于2025-09-23 15:19:57
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Mo-doped Zn, Co Zeolitic-Imidazolate Framework-derived Co9S8 Quantum Dots and MoS2 Embedded in Three-Dimensional Nitrogen Doped Carbon Nano???ake Arrays as an Efficient Trifunctional Electrocatalysts for ORR, OER and HER
摘要： Herein, we first propose a facile strategy to synthesize Co9S8 and MoS2 nanocrystals embedded in porous carbon nanoflake arrays supported on carbon nanofibers (Co9S8-MoS2/N-CNAs@CNFs) by the pyrolysis of Mo-doped Zn, Co zeolitic-imidazolate framework grown on carbon nanofibers and subsequent sulfuration. The electrocatalyst shows high and stable electrocatalytic performance, with half-wave potential of 0.82 V for ORR and overpotential at 10 mA cm-2 for OER (0.34 V) and HER (0.163 V), which outperform the metal-organic frameworks-derived transition metal sulfide catalysts reported so far. Furthermore, the Co9S8-MoS2@N-CNAs@CNFs are employed as an air cathode in a liquid-state and all-solid-state zinc-air battery, presenting high power density of 222 mW cm-2 and 96 mW cm-2, respectively. Such excellent catalytic activities are mainly owing to the unique three-dimensional structure and chemical compositions, optimal electronic conductivity, adequate surface area and the abundance of active sites. Thus, this work provides an important method for designing other metal-organic frameworks derived three-dimensional structural sulfide quantum dot multifunctional electrocatalyst for wider application in highly efficient catalysis and energy storage.
关键词： zeolitic-imidazolate framework,Co9S8 quantum dots,MoS2,nitrogen-doped carbon nanoflakes arrays,Zn-air battery,trifunctional electrocatalysts
更新于2025-09-23 15:19:57
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High-Efficiency Perovskite Solar Cells Enabled by Anatase TiO2 Nanopyramid Arrays with Oriented Electric Field
摘要： One-dimensional (1D) nanostructured oxides have been proposed as excellent electron transport materials (ETMs) for perovskite solar cells (PSCs), but this has not yet been demonstrated experimentally. Here, we exploit a facile hydrothermal approach to grow highly oriented anatase TiO2 nanopyramid arrays and further demonstrate their advantages for application in PSCs. The oriented TiO2 nanopyramid arrays afford sufficient contact area for electron extraction and increase light transmission. Moreover, the nanopyramid array/perovskite system exhibits an oriented electric field that can increase charge separation and accelerate charge transport, thereby suppressing charge recombination. As a result, the anatase TiO2 nanopyramid arrays-PSCs deliver a champion power conversion efficiency of ~22.5%, which is the highest PCE reported thus far for PSCs consisting of 1D ETMs. This work demonstrates that the rational design of 1D ETMs can achieve PSCs that perform as well as typical mesoscopic and planar PSCs.
关键词： Anatase TiO2,Electric field distribution,Perovskite solar cells,One-dimensional nanostructures,Nanopyramid arrays
更新于2025-09-23 15:19:57
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Metasurfaces: Subwavelength nanostructure arrays for ultrathin flat optics and photonics
摘要： Miniaturization is a strong demand of modern scientific technology. However, conventional optical components based on refraction suffer from functional degradation as the device size decreases. Metasurfaces consisting of subwavelength optical antenna arrays have emerged as planar optical devices that enable many promising applications in lenses, holograms, and optical cloaks. During recent decades, metasurfaces have been developed for their specific functionalities by exploiting new materials and design algorithms. In this issue of MRS Bulletin, progress in metasurfaces is discussed to provide a comprehensive understanding of metasurfaces and their novel applications in optics and photonics.
关键词： subwavelength nanostructure arrays,photonics,Metasurfaces,ultrathin flat optics
更新于2025-09-23 15:19:57
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Dye-sensitized solar cells based on TiO2 nanoparticles-decorated ZnO nanorod arrays for enhanced photovoltaic performance
摘要： Herein, we report a successful approach for the vertically aligned ZnO nanorod arrays (ZNAs) deposited on fluorine-doped tin oxide (FTO) substrate by hydrothermal process. TiO2 nanoparticles were grown on the ZNAs by dip-coating. ZNAs and TiO2 nanoparticles (TNPs)-decorated ZNAs (TNPs@ZNAs) were used as a photoanode in dye-sensitized solar cells. The influence of bath temperature for the attainment of uniform decoration of TiO2 nanoparticles onto ZnO nanorod arrays and the photovoltaic performances of the assembled dye-sensitized solar cells were studied. The power conversion efficiency (PCE) of the TNPs@ZNAs arrays prepared at a bath temperature of 120 °C can reach 4.47%, representing better improvement when compared with ZNAs photoanode (3.15%).
关键词： Nanorod arrays,Bath temperature,Dye-sensitized solar cells,TiO2 decorated ZnO
更新于2025-09-23 15:19:57
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[IEEE 2018 11th UK-Europe-China Workshop on Millimeter Waves and Terahertz Technologies (UCMMT) - HangZhou, China (2018.9.5-2018.9.7)] 2018 11th UK-Europe-China Workshop on Millimeter Waves and Terahertz Technologies (UCMMT) - High-Efficiency Transmission-Type Digital Coding Metasurface for Metalens and Transmitarray
摘要： Field-programmable gate arrays (FPGAs) have been shown to provide high computational density and efficiency for many computing applications by allowing circuits to be customized to any application of interest. FPGAs also support programmability by allowing the circuit to be changed at a later time through reconfiguration. There is great interest in exploiting these benefits in space and other radiation environments. FPGAs, however, are very sensitive to radiation and great care must be taken to properly address the effects of radiation in FPGA-based systems. This paper will highlight the effects of radiation on FPGA-based systems and summarize the challenges in deploying FPGAs in such environments. Several well-known mitigation methods will be described and the unique ability of FPGAs to customize the system for improved reliability will be discussed. Finally, two case studies summarizing successful deployment of FPGAs in radiation environments will be presented.
关键词： radiation effects,radiation hardening,field programmable gate arrays,integrated circuit reliability,Fault-tolerant systems
更新于2025-09-23 15:19:57
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The Inspection of CFRP Laminate with Subsurface Defects by Laser Arrays Scanning Thermography (LAsST)
摘要： Laser array scanning thermography (LAsST) was used to detect the subsurface defects of carbon fiber reinforced composite (CFRP). A series of bottom flat hole (BFHs) of CFRP were prepared for LAsST. Truncation pseudo-static matrix reconstruction (TC-PSMR) method was used to reconstruct the thermal response signal. Fast Fourier transform (FFT), principal component analysis (PCA) and partial least squares regression (PLSR) were used to process the thermal response signals, forming FFT image, PCA image, and PLSR image. The signal noise ratios (SNRs) of defects is calculated, and it is used to evaluate the defect detection ability of different post-processing algorithms. The experimental results show that the image based on FFT phase has a higher signal-to-noise ratio with PLSR image, and the FFT amplitude image and PLSR image can accurately represent the defect size.
关键词： FFT,Laser arrays scan thermography,Partial least squares regression,CFRP
更新于2025-09-23 15:19:57
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Ferroelectric properties and phase transitions of high performance vertically aligned KNN nanowire-arrays grown by pulsed laser deposition
摘要： Pulsed laser deposition (PLD) was used to synthesize piezoelectric nanowire-arrays of K0.5Na0.5NbO3 (KNN) on Pt/TiO2/SiO2/Si substrates. These arrays were successfully prepared by using two different deposition conditions than the previously reported for KNN. KNN with orthorhombic structure and minority secondary phases were identified by XRD. Ferroelectric and Piezoelectric properties were confirmed by piezoresponse force microscopy, and showed that nanowire-arrays have an improvement in their effective piezoelectric coefficient of d33eff = 94.6 pm/V and 133.6 pm/V, higher than previously reported coefficients. Pulsed laser photoacoustic technique was used to analyze the phase transition temperatures and they showed a phase transition (O-T) at ～170 ?C and a phase transition (T-C) at ～360 ?C, lower temperatures than those found for bulk ceramics. Furthermore, it was identified the presence of minor amount of secondary ferroelectric phase (K4Nb6O17).
关键词： Phase transitions,KNN nanowire-arrays,Ferroelectric properties,Pulsed laser deposition,Piezoelectric coefficient
更新于2025-09-23 15:19:57
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Lab-on-Fiber: Plasmonic Nano-arrays for Sensing
摘要： For sensors based on electromagnetic resonance whether surface plasmon resonance (SPR) or localized surface plasmon resonance (LSPR), enhancing the light-matter interactions is the most critical and important way to improve the performance of sensors. Plasmonic nano-arrays is a kind of periodic metal or dielectric nanostructure formed by nanofabrication technology and it can effectively enhance the light-matter interactions by tuning structural parameters to excite different optical effects due to its ultra-high degree of freedom. At the same time, a plug-and-play, remote micro sensor suitable for limited environments (such as in vivo) may be realized due to the rise of lab-on-fiber technology and the progress of nanofabrication technology for unconventional substrates (such as optical fiber tip). In this paper, the advantages and disadvantages of different nanofabrication technologies are briefly introduced and compared firstly, and then the applications of optical fiber sensors (OFS) based on different plasmonic nano-arrays are reviewed. Plasmonic nano-arrays OFS are divided into two categories: one is the refractive index sensor based on the sensitivity of the array to the surrounding environment; the other is the surface enhanced Raman scattering (SERS) sensor based on the enhancement ability of the local electric field around the array. In this review, the present sensors are compared and analyzed from aspects of the geometry, material and dimension of plasmonic nano-arrays and the main research directions and progress are summarized. Finally, the future development trend is proposed.
关键词： surface plasmon resonance,localized surface plasmon resonance,optical fiber sensors,nanofabrication technologies,Plasmonic nano-arrays,lab-on-fiber
更新于2025-09-23 15:19:57
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[IEEE 2019 IEEE 13th International Conference on Power Electronics and Drive Systems (PEDS) - Toulouse, France (2019.7.9-2019.7.12)] 2019 IEEE 13th International Conference on Power Electronics and Drive Systems (PEDS) - Sizing and Control of a Multilevel Converter for Photovoltaic Generation with Independent Power Extraction Capabilities per Module
摘要： One of the main vulnerabilities of GNSS receivers jamming is their exposure to intentional or unintentional signals, which could even cause service unavailability. Several alternatives to counteract these effects were proposed in the literature, being the most promising those based on multiple antenna architectures. This is specially the case for high-grade receivers used in applications requiring reliability and robustness. This article provides an overview of the possible receiver architectures encompassing antenna arrays and the associated signal processing techniques. Emphasis is also put on the most typical implementation issues found when dealing with such technology. A thorough survey is complemented with a set of experiments, including real data processing by a working prototype, which exemplifies the above ideas.
关键词： electromagnetic interference,receiving antennas,robustness,radio navigation,availability,satellite navigation systems,Adaptive arrays,array signal processing,global positioning system
更新于2025-09-23 15:19:57