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Impact of dielectric environment on the linear and nonlinear optical properties for CdS/ZnS cylindrical core/shell quantum dots
摘要： By the mean of the effective mass approximation (E.M.A) and compact density matrix method, the energy eigenvalues, linear and nonlinear dielectric function have been theoretically investigated for CdS/ZnS cylindrical core/shell quantum dot embedded in PVA, PMMA and SiO2 matrices. Simulation results showed that the presence of the dielectric mismatch in the QD-matrix system can lead to a significant enhancement of the nonlinear dielectric function. According to our calculations, peaks of the real and imaginary part of the dielectric function can experience a redshift or a blue shift with the appropriate dielectric environment.
关键词： complex dielectric function,Effective mass approximation,cylindrical core/shell quantum dot,density matrix approach
更新于2025-09-23 15:19:57
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Dielectric environment effect on linear and nonlinear optical properties for CdS/ZnS core/shell quantum dots
摘要： The eigenvalues, transition energy, the linear and nonlinear dielectric functions have been numerically investigated for CdS/ZnS spherical core/shell quantum dots embedded in various dielectric matrices. The evaluation was carried out for three commonly used matrices, such as PVA, PMMA and SiO2. Calculations were done under the effective mass approximation and compact density matrix approach. Results revealed that the nonlinear optical property is strongly affected by the nature of the matrix material. By increasing core/shell radii ratio the energy states as well as the transition energy are decreasing. It is also indicated that the presence of the dielectric mismatch in the QD-matrix system can cause significant enhancement on the linear and third order nonlinear dielectric function.
关键词： Complex dielectric function,Core/shell,Density matrix approach,Effective mass approximation,Nonlinear optic
更新于2025-09-12 10:27:22