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Spectral splitting and phase matching of the macroscopic high-order harmonic generation in intense laser fields
摘要： We theoretically investigate the macroscopic high-order harmonic generation in argon gaseous medium by numerically solving the three-dimensional macroscopic propagation equation, and the results show that the harmonic spectral and spatial profiles of harmonics are gradually splitting with the increasing of the driving laser intensity. This splitting is mainly due to the distortions which the driving field suffers during propagation and the consequence is also on phase matching. To illustrate the physical mechanisms of harmonic splitting, a theoretical analysis of the phase matching is presented. The harmonic spectra from different focus positions reveal that the split is dependent on the focus-gas-jet relative position. Moreover, we demonstrate that the spectral splitting of high harmonics can hardly be observed for neon gas jet due to the high ionization energy.
关键词： phase matching,high-order harmonic generation,intense laser fields,macroscopic propagation,spectral splitting
更新于2025-09-23 15:19:57
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Ultrafast Structural Dynamics of Nanoparticles in Intense Laser Fields
摘要： Femtosecond laser pulses have opened new frontiers for the study of ultrafast phase transitions and nonequilibrium states of matter. In this Letter, we report on structural dynamics in atomic clusters pumped with intense near-infrared (NIR) pulses into a nanoplasma state. Employing wide-angle scattering with intense femtosecond x-ray pulses from a free-electron laser source, we find that highly excited xenon nanoparticles retain their crystalline bulk structure and density in the inner core long after the driving NIR pulse. The observed emergence of structural disorder in the nanoplasma is consistent with a propagation from the surface to the inner core of the clusters.
关键词： x-ray scattering,nanoparticles,nanoplasma,intense laser fields,ultrafast structural dynamics
更新于2025-09-11 14:15:04