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Porous Organic Polymer-Coated Band-Aids for Phototherapy of Bacteria-Induced Wound Infection
摘要： Band-Aids have been widely used for wound care. For most adhesive bandages, however, they have limited capacity to speed up the wound healing process, which in turn may cause serious wound infections. In this study, antibacterial Band-Aids, combining porphyrin based porous organic polymers (POPs) with commercial antibiotics-free Band-Aids, are designed. Under white light irradiation, POP can produce effective photothermal heat, as well as highly reactive oxygen species (ROS), thereby triggering the potent hyperthermia and simultaneous ROS increase on wounds. What's more, white-light is similar with sunlight, which makes POP-based Band-Aids (PBA) ideal wound dressings for wound disinfection.
关键词： wound infection,porous organic polymers,band-aids,white light
更新于2025-09-23 15:23:52
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End-pump high efficiency 355 nm laser with a convex–concave cavity and optically-uncoated Brewster angle-cut LiB <sub/>3</sub> O <sub/>5</sub> crystal
摘要： Porous organic polymers (POPs), with features of permanent nanopores and designable frameworks, show great promise as sulfur host materials to restrain the shuttling of polysulfides, one of the main obstacles in the development of lithium–sulfur batteries. However, the simple physical entrapment from weak intermolecular interactions via a typical melt-diffusion method results in the diffusive loss of polysulfides that has thus far restricted their potential. Herein, a facile strategy for introducing chemical covalent interactions between POPs and sulfur via the regulation of sulfur infiltration temperature is reported. The results show that increasing the temperature to a suitable value, e.g., 400 °C, for a fluorinated triazine-based framework (FCTF), enables chemical bonding between the sulfur and aromatic FCTF backbone. Benefitting from the synergetic chemical and physical confinement effect, the shuttling of polysulfides can be efficiently restrained. As a result, the sample features superior sulfur utilization, high-rate performances, and good cycle stability, as compared with the sample with only physical confinement. The proposed strategy can also be extended to other POPs, such as the boroxine-linked covalent organic framework, by judiciously tailoring the infiltration temperatures. The findings disclose the important role of infiltration temperatures in developing efficient cathode host materials for lithium–sulfur batteries.
关键词： porous organic polymers,electrochemical performance,covalent chemical interactions,lithium–sulfur batteries,elevated sulfur infiltration temperature
更新于2025-09-11 14:15:04