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Climatological analysis of the optical properties of aerosols and their direct radiative forcing in the Middle East
摘要： In addition to climate perturbations, various problems such as air pollution, reduction in the visibility and human health hazards were caused by atmospheric aerosols in the Middle East specifically in the last two decades. With the help of the Aerosol Robotic NETwork (AERONET), the measurement of the aerosol optical and radiative properties were carried out over seven sites in the Middle East during 2013. The analysis of the optical properties of aerosols like Single Scattering Albedo (SSA), Angstrom Exponent (AE), Aerosol Optical Depth (AOD), and Asymmetry parameter (ASY) were carried out during the study period. During spring and summer, high values of AOD and low values of AE were found in all sites except CUT-TEPAK (Limassol, Cyprus), which specified the existence of coarse mode particles and dust storms in these seasons. The AE maximum values were found in the summer and fall over CUT-TEPAK and IMS-METU-ERDEMLI(Erdemli, Turkey), whereas in other sites IASBS (Zanjan, Iran), KAUST Campus (Thuwal, Saudi Arabia), Masdar Institute (Masdar, United Arab Emirates), Mezaira (Mezaira, United Arab Emirates) and Solar Village (Riyadh, Saudi Arabia) the peak values of AE occurred in the fall and winter. The maximum values of SSA and ASY were observed in the spring and summer over all sites except over CUT-TEPAK and IMS-METU-ERDEMLI. The Santa Barbara DISORT Atmospheric Radiative Transfer (SBDART) model has been used for the calculations of the Aerosol Radiative Forcing (ARF) over the selected sites. We obtained negative value of ARF at the surface, which suggesting its cooling effects because of the loss of radiation back to space due to aerosols. The averaged ARF values at the SuRFace (SRF) of the earth were -43.8 Wm-2, -31 Wm-2, -56.8 Wm-2, -61.7 Wm-2, -52.5 Wm-2, -54.9 Wm-2, and -72.2 Wm-2, over CUT-TEPAK, IASABS, IMS-METU-ERDEMLI, KAUST Campus, Masdar Institute, Mezaira and Solar Village, respectively. While the positive value of atmospheric ARF showed heating of the atmosphere.
关键词： Middle East.,Aerosol Optical Depth,SBDART,Aerosol Radiative Forcing,AERONET
更新于2025-09-23 15:23:52
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A 10-year record of aerosol optical properties and radiative forcing over three environmentally distinct AERONET sites in Kenya, East Africa
摘要： In the framework of Aerosol Robotic Network (AERONET), the aerosol optical, microphysical and radiative properties were investigated over three sites (CRPSM_Malindi, Nairobi, and ICIPE_Mbita) in Kenya, East Africa (EA) during 2006-2015. The annual mean (±σ) aerosol optical depth at 440 nm (AOD440) was found high at Mbita (0.27±0.09) followed by Malindi (0.26±0.07), and low at Nairobi (0.19±0.04). Whereas, the seasonal mean AOD440 noticed high (low) values during the local dry (wet) seasons. The aerosol optical properties: AOD, single scattering albedo (SSA), asymmetry parameter (ASY), and complex aerosol refractive index (RI) exhibited significant temporal and spectral heterogeneities illustrating the complexity of aerosol types with an abundance of fine-mode aerosols during the local dry (JJA) season. Characterization of major aerosol types revealed the dominance of mixed-type followed by biomass burning aerosols. The aerosol volume size distribution revealed that the coarse- over fine-mode aerosols showed a significant contribution to the total volume particle concentration, especially at high (> 0.3) AOD440. Further, the aerosol columnar number size distribution (CSD) retrieved from the King’s inversion of spectral AOD exhibited a power law distribution affirming multiplicity of aerosol sources. The direct aerosol radiative forcing values simulated in the shortwave region using the Santa Barbara DISORT Atmospheric Radiative Transfer (SBDART) model showed good correlation (r=>0.85) with the AERONET derived ones at the top-of-atmosphere (TOA), bottom-of-atmosphere (BOA) and within the atmosphere (ATM). The annual mean (±σ) TOA, BOA, and ATM forcing values were found in the range from -8.10±3.75 to -13.23±4.87, -34.54±4.86 to -46.11±10.27, and 26.63±6.43 to 36.24±7.26 Wm-2, respectively, with an atmospheric heating rate (AHR) of 0.74±0.12–1.02±0.20 K day-1. The SBDART-derived DARF exhibited significant temporal heterogeneity with high (low) during the local dry (wet) seasons. Results derived from the present study forms a basis for regional climate change studies and could increase the accuracy of climate models over this unexplored region of Africa.
关键词： Aerosol radiative forcing,Aerosol optical depth,Size distribution,East Africa,AERONET,Single scattering albedo
更新于2025-09-23 15:22:29
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Impacts of distribution patterns of cloud optical depth on the calculation of radiative forcing
摘要： The gridding process applied to satellite-retrieved cloud properties results in the loss of certain information. In this study, we analyzed the error associated with using gridded cloud optical depth (τ) in calculating radiative forcing from the perspective of the distribution pattern of τ. Utilizing the simulated results from SBDART (Santa Babara DISORT Atmospheric Radiative Transfer), we calculated this error in ideal probability distribution functions (PDFs) of τ while keeping the average τ constant, and then used the τ retrieved from MODIS (Moderate Resolution Imaging Spectroradiometer) pixel-level observations to simulate real case studies. The results from both the ideal experiments and real case studies indicate that there is a large dependence of the error caused by gridding process on the PDF of τ. The greatest relative error occurs in the cases when τ fits a two-point or uniform distribution, reaching 10–20%, while this error is below 5% when τ follows a binomial distribution. From the analysis of MODIS pixel-level data from June 2016, we found that the PDFs of τ within one grid point (1° × 1°) could not be simply described by a normal distribution. Although using the logarithmic mean of τ controls the error effectively, the error can still be up to 4%. Our study suggests that using gridded data (especially the arithmetic mean) to calculate radiative forcing may result in uncertainty to a certain extent, which depends strongly on the distribution pattern of cloud properties within the grid point. The PDF of cloud properties should be comprehensively considered in the gridding process in the future.
关键词： Radiative forcing,Distribution pattern,Cloud optical depth,Grid,MODIS
更新于2025-09-19 17:15:36
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Light absorption by organic aerosol emissions rivals that of black carbon from residential biomass fuels in South Asia
摘要： Solid biomass fuel-based residential cookstoves are the largest source of aerosol emissions in the Indian subcontinent. For assessing radiative forcing due to this pollutant source, laboratory-generated cookstove performance datasets are currently used, which have established black carbon (BC) as the dominant atmospheric warming aerosol species. We report findings on the strong near-ultraviolet wavelength absorption characteristics of emitted organic carbon (OC) aerosol from household stove combustion of nationally-representative biomass fuels. OC emission from cookstoves have been conventionally parameterized in emission inventory and regional climate models to be non-light-absorbing in the visible solar spectra. We conclude that light-absorbing OC contributes roughly as much as BC to total absorption cross-sections, thereby enhancing the associated positive forcing estimates. Our findings underscore the importance of including light-absorbing OC within the subcontinent’s air quality and climate impact assessment frameworks.
关键词： South Asia,black carbon,radiative forcing,biomass fuels,organic carbon,light absorption,cookstoves,aerosol emissions
更新于2025-09-19 17:13:59
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Case study of spatial and temporal variability of snow cover, grain size, albedo and radiative forcing in the Sierra Nevada and Rocky Mountain snowpack derived from imaging spectroscopy
摘要： Quantifying the spatial distribution and temporal change in mountain snow cover, microphysical and optical properties is important to improve our understanding of the local energy balance and the related snowmelt and hydrological processes. In this paper, we analyze changes of snow cover, optical-equivalent snow grain size (radius), snow albedo and radiative forcing by light-absorbing impurities in snow and ice (LAISI) with respect to terrain elevation and aspect at multiple dates during the snowmelt period. These snow properties are derived from the NASA/JPL Airborne Visible/Infrared Imaging Spectrometer (AVIRIS) data from 2009 in California’s Sierra Nevada and from 2011 in Colorado’s Rocky Mountains, USA.
关键词： snow cover,grain size,Sierra Nevada,Rocky Mountains,imaging spectroscopy,radiative forcing,albedo
更新于2025-09-04 15:30:14