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Angular streaking of Auger-electrons by THz field
摘要： Rotational streaking by a circularly polarized THz field of Auger electrons generated by a short extreme ultraviolet (XUV) or X-ray pulse is theoretically investigated. The character of the streaking pattern depends on three main parameters: the duration of the XUV pulse, the Auger decay time-of-life and the period of the THz field. Different cases with various interrelations of these parameters are discussed. Examples of the patterns are calculated within the strong field approximation. Correspondence between the angular streaking of electrons in the processes of photoionization and Auger ionization is considered. Retrieval of the Auger decay parameters from circular streaking spectrum is discussed.
关键词： THz field,strong field approximation,Auger electrons,angular streaking,ultrafast processes
更新于2025-09-23 15:23:52
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Dynamical distortions of structural signatures in molecular high-order harmonic spectroscopy
摘要： We study the signature of two-center interferences in molecular high-order harmonic spectra, with an emphasis on the spectral phase. With the help of both ab initio computations based on the time-dependent Schr?dinger equation and the molecular strong-field approximation (SFA) as developed by Chiril? et al. [Phys. Rev. A 73, 023410 (2006)] and Faria [Phys. Rev. A 76, 043407 (2007)], we observe that the phase behavior is radically different for the short and the long trajectory contributions. By means of Taylor expansions of the molecular SFA, we link this effect to the dynamics of the electron in the continuum. More precisely, we find that the value of the electric field at recombination time plays a crucial role in the shape of the destructive interference phase jump.
关键词： molecular spectroscopy,spectral phase,strong-field approximation,two-center interferences,time-dependent Schr?dinger equation,high-order harmonic generation
更新于2025-09-23 15:23:52