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Generation of optical signal and terahertz idler photons by spontaneous parametric down-conversion
摘要： Frequency-angular characteristics of signal and idler photons generated under spontaneous parametric down-conversion are studied in a strongly frequency nondegenerate regime, without paraxial approximation, accounting for possible inherent absorption of idler waves in a nonlinear crystal, classical thermal field fluctuations, and the multimode character of parametric interaction induced by transverse spatial limitation of the pump beam. Spatial limitation is shown to lead to a huge increase in angular divergence of the idler photons generated at terahertz frequencies. General expressions are obtained for the frequency-angular sensitivity function of the nonlinear-optical terahertz wave detector and for power densities of the signal and idler photon fluxes. The absorption-induced difference in the parametric conversion coefficients for the noise and externally incident radiation of the idler frequency is shown to be described by approximately the same loss factor for all active spatial idler modes. Two different parametric contributions of the internal thermal noise to the number of output idler photons were revealed with different dependence on the idler-wave absorption. Expressions for the loss factors, which describe absorption-induced effects in signal and idler channels, are obtained and shown to be turning into one another by changing the sign of the absorption coefficient. Relative contribution of thermal and quantum field fluctuations into the intrinsic radiation of a nonlinear crystal at signal and idler frequencies is analyzed accounting for the crystal absorption properties.
关键词： nonlinear optics,thermal fluctuations,terahertz,quantum fluctuations,absorption,spontaneous parametric down-conversion
更新于2025-09-23 15:22:29
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Indirect tail states formation by thermal-induced polar fluctuations in halide perovskites
摘要： Halide perovskites possess enormous potential for various optoelectronic applications. Presently, a clear understanding of the interplay between the lattice and electronic effects is still elusive. Specifically, the weakly absorbing tail states and dual emission from perovskites are not satisfactorily described by existing theories based on the Urbach tail and reabsorption effect. Herein, through temperature-dependent and time-resolved spectroscopy on metal halide perovskite single crystals with organic or inorganic A-site cations, we confirm the existence of indirect tail states below the direct transition edge to arise from a dynamical Rashba splitting effect, caused by the PbBr6 octahedral thermal polar distortions at elevated temperatures. This dynamic effect is distinct from the static Rashba splitting effect, caused by non-spherical A-site cations or surface induced lattice distortions. Our findings shed fresh perspectives on the electronic-lattice relations paramount for the design and optimization of emergent perovskites, revealing broad implications for light harvesting/photo-detection and light emission/lasing applications.
关键词： thermal fluctuations,halide perovskites,Rashba effect,optoelectronics,tail states
更新于2025-09-19 17:15:36
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[IEEE 2019 Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC) - Munich, Germany (2019.6.23-2019.6.27)] 2019 Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC) - Thermal Noise in Optically Pumped DF-VECSELs
摘要： Over the last decades, the low noise properties of Vertical–External–Cavity Surface–Emitting Lasers (VECSELs) have aroused interest for various applications. The dual–frequency (DF) VECSELs can generate a very low noise RF signal resulting from the beatnote of two orthogonal linear polarizations as sketched in Fig.1(a). For example, the very high spectral purity and class–A operation of DF–VECSELs are of interest for ultrastable atomic clocks [1] or microwave electronics for optically-carried RF signal processing or wide-band RADARs. The sources of noise of optically pumped VECSELs are well identi?ed : (i) the intensity noise induced by the pump through the laser dynamics, (ii) the spontaneous emission contribution, (iii) technical noises such as mechanical vibrations, and (iv) the thermal noise. The two ?rst sources of noise are well modeled and understood. But in [2] a simple second–order low-pass ?lter behaviour is assumed for the thermal contribution to the frequency noise power spectral density (PSD) spectra. Yet, de?ning unequivocally a cut–off frequency is not obvious since different time scales are actually involved. Moreover, this over–simpli?ed model fails at low frequencies in [3] as displayed in Fig.1(b). Indeed, below 200 kHz the slope of the beatnote phase–noise spectrum of a DF–VECSEL at 852 nm obeys a f ?3 scaling law instead of the f ?4 expected behaviour. The aim of the present work is to microscopically model the thermal noise contribution. First, we describe the layers of the optically pumped emitting–surface, which is glued to a Peltier cooler. The heat equations take into account transverse and longitudinal diffusion processes. Assuming a gaussian pro?le for the pump, we obtain the temperature ?eld inside the structure using Hankel transformation formalism and we investigate the transient thermal response. The pump intensity ?uctuations induce heat ?uctuations inside the structure leading to changes of the refractive index and the material thermal–expansion, which are responsible for frequency ?uctuations of the laser mode. We ?nd an analytical expression of the frequency noise PSD induced by these thermo-optic effects, which allows to model the beatnote phase noise PSD of DF-VECSELs. We ?nd a very good agreement with the f ?3 slope of the experimental datas and we evidence the fundamental thermal ?uctuations contribution at room temperature. Such thermodynamics ?uctuations were already investigated for VCSEL structures in [4], starting from a stochastic heat equation. We extend it to a full study of the frequency noise PSD spectrum for DF-VECSELs. We obtain a fully analytical expression and discuss its validity.
关键词： Thermal noise,frequency noise PSD,thermal fluctuations,optically pumped,DF-VECSELs
更新于2025-09-16 10:30:52