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1D ballistic transport channel probed by invasive and non-invasive contacts
摘要： Epitaxially grown sidewall graphene nanoribbons show a robust quantum conductance of e2/h. By means of in-situ transport measurements with a nanoprobe system, we realized invasive and non-invasive 4-point-probe configurations. The invasiveness correlates with the contact resistance of the voltage probes. In particular, we achieved now non-invasive voltage probes revealing an almost zero resistance in a collinear 4 point-probe measurement. This proofs the ballistic nature of our epitaxially grown sidewall nanoribbons on SiC(0001) mesa structures.
关键词： quantum conductance,graphene nanoribbons,ballistic transport,non-invasive contacts,invasive contacts
更新于2025-09-23 15:21:21
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Photoelectron Spectroscopy of Molecular Anion of Alq <sub/>3</sub> : An Estimation of Reorganization Energy for Electron Transport in the Bulk
摘要： A molecular anion of tris(8-hydroxyquinolinato)aluminum (Alq3) was generated by a pulsed discharge to the solid sample under supersonic expansion and its photoelectron spectrum was recorded after mass selection. The vertical detachment energy of Alq3? and the adiabatic electron affinity of Alq3 were determined to be 1.24 ± 0.01 and 0.89 ± 0.04 eV, respectively. By using these energies determined for monomeric Alq3, the reorganization energy for the intermolecular electron transport in bulk Alq3 was estimated to be 0.70 ± 0.08 eV.
关键词： Photoelectron Spectroscopy,Electron Transport,Reorganization Energy,Alq3,Molecular Anion
更新于2025-09-23 15:21:21
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Nonradiative decay and absorption rates of quantum emitters embedded in metallic systems: Microscopic description and their determination from electronic transport
摘要： We investigate nonradiative decay and absorption rates of two-level quantum emitters embedded in a metal at low temperatures. We obtain the expressions for both nonradiative transition rates and identify a unique, experimentally accessible way to obtain both nonradiative transition rates via electronic transport in the host metallic system. Our findings not only provide a microscopic description of the nonradiative channels in metals, but they also allow one to identify, determine, and differentiate them from other decay channels, which is crucial to the understanding and controlling of the light-matter interactions at the nanoscale.
关键词： nonradiative decay,metallic systems,quantum emitters,electronic transport,absorption rates
更新于2025-09-23 15:21:21
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Low Frequency Dielectric Relaxation and Charge Transport in Bi<sub>12</sub>TiO<sub>20 </sub>Photorefractive Sillenite Crystals
摘要： Features of processes of a dielectric relaxation and charge transport in photorefractive sillenite crystals Bi12TiO20 at low frequency range are investigated. It was found that the dispersion of dielectric permittivity ε' in crystals Bi12TiO20 is characterized by its growth with lowering frequency and rising temperature. This behaviour may be related to existence of dipole-relaxation polarization mechanism. The frequency dependence of dielectric loss tgδ reveals the existence of low frequency relaxation peaks in the studied temperature range. From the conductivity dependence on the frequency and temperature it was found that conductivity σ increases as frequency increases in the low frequency range. The observed dependence σ(ω)≈Аωs indicates that transport mechanism is due to hopping of carriers via localized electron states. The charge transport is thermally activated process in which activation energy Ea = (0.82±0.03) eV.
关键词： Charge transport,Photorefractive Sillenite crystals,Dielectric relaxation
更新于2025-09-23 15:21:21
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[IEEE 2018 31st International Vacuum Nanoelectronics Conference (IVNC) - Kyoto, Japan (2018.7.9-2018.7.13)] 2018 31st International Vacuum Nanoelectronics Conference (IVNC) - Field emission from Au nanoparticles decorated ZnO nanowires
摘要： ZnO nanowires with Au nanoparticle decoration were prepared. Photoluminescence results reveal quenching of both the band edge and visible emissions of ZnO nanowires after the Au nanoparticle decoration. The field emission properties fro\ Au nanoparticles decorated ZnO nanowires were measured and increasing turn-on fields were observed. The observed phenomena were attributed to electron transport between ZnO and Au nanoparticle.
关键词： ZnO nanowires,Au nanopartical,field-emisison,electron transport
更新于2025-09-23 15:21:21
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[IEEE 2018 31st International Vacuum Nanoelectronics Conference (IVNC) - Kyoto, Japan (2018.7.9-2018.7.13)] 2018 31st International Vacuum Nanoelectronics Conference (IVNC) - Nanogranular Compound Material Layers Serve as Storage for Infra-red to Ultra-Violet Photons for the Energy Supply for Electric Machines
摘要： Hyper-Giant conducting nanogranular compound materials, which serve as IR photon detectors allow to use BOSON-current transport at room temperature with GA/cm2 current carrying capability for Energy applications
关键词： Room temperature,Bosons having parallel spin,Boson-current transport,Energy supply for electric machines
更新于2025-09-23 15:21:21
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Electronic transport induced by edge modification of graphene electrodes in single molecular device
摘要： The aim was to study the electronic transport of molecular devices constructed by salicylidene aniline molecule and graphene electrodes using the density functional theory and non-equilibrium Green’s function. The calculated results demonstrate a switching behavior in two photoisomerizations. In addition, the modification of –OH on the edge of graphene nanoribbons induces the variety of the frontier molecular orbitals and the increase of current, but the decrease of switching ratio. The modification of F on the edge of graphene nanoribbons improves the switching ratio. We explain the negative differential resistance effect found in the device by transmission spectra and the evolution of local density of states at the bias. The results indicate that different modifications on the edge of graphene nanoribbons influence the electronic transport. This method can improve the application of the device in future molecular circuits.
关键词： Electronic transport,Edge modification,Molecular switching
更新于2025-09-23 15:21:21
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First-principle studies on electron transport properties in four-terminal MoS2 nanoribbons
摘要： We perform the ?rst-principle studies on electron transport through four-terminal MoS2 nanoribbons. It is found that in such structures, insulating bands exist in the linear-conductance spectra of the nanoribbons with straight channels, which are related to the band gaps of the MoS2 nanoribbons. However, nonzero transports are allowed to take place in the insulating-band region in the geometries with curved channels. This phenomenon can be attributed to the formation of edge states in the curved-channel structures. We believe that these results provide useful information for the manipulation of electron transport through MoS2 nanoribbons.
关键词： Electron transport,First-principle studies,MoS2 nanoribbons
更新于2025-09-23 15:21:21
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Mechanism of Liquid-Phase Reductive Thin-Film Deposition under Quasiballistic Electron Incidence
摘要： Highly reducing activity of quasiballistic hot electrons emitted from a nanocrystalline silicon (nc-Si) diode is veri?ed in terms of liquid-phase thin ?lm deposition. Incident electrons reduce positive ions in salt solutions coated on a target substrate, and then result in deposition of thin metal (Cu) and semiconducting (Si, Ge, and SiGe) ?lms. This mechanism is investigated here throughout the process from electron incidence to thin ?lm deposition. Thermodynamic criterion deduced from classical nucleation theory suggests that the output electron energy of the nc-Si emitter is suitable for promoting preferential reduction of target ions in solutions leading to the nuclei formation. In accordance with mass-transport analyses on generated nanoclusters, the most primary factor of thin ?lm growth is the dose of incident electron. The formulated deposition rate rapidly increases and reaches a stationary value within 0.1 s after electron incidence. The theoretical dependency of the thin ?lm thickness on the electron incidence time is consistent with the experimental results. Speci?c features of this scheme as an alternative approach for thin ?lm deposition are discussed in comparison with the conventional dry and wet processes.
关键词： nanocrystalline silicon diode,quasiballistic hot electrons,mass-transport analyses,thermodynamic criterion,liquid-phase thin film deposition
更新于2025-09-23 15:21:21
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Formation of Occupied and Unoccupied Hybrid Bands at Interfaces between Metals and Organic Donors/Acceptors
摘要： Efficient charge transport in organic semiconductors and at their interfaces with electrodes is crucial for the performance of organic molecule-based electronic devices. Band formation fosters effective transport properties and can be found in organic single crystals of large π-stacking aromatic molecules. However, at molecule/metal interfaces hybrid band formation and band dispersion is a rarely observed phenomenon. Using angle-resolved two-photon photoemission supported by density functional theory calculations we demonstrate such band formation for two different molecule/metal systems, namely tetrathiafulvalene (TTF)/Au(111) and tetrafluoro-tetracyanoquinodimethane (F4TCNQ)/Au(111), in the energy region of occupied as well as unoccupied electronic states. In both cases strong adsorbate/substrate interactions result in formation of interface states due to hybridization between localized molecular states and delocalized metal bands. These interface states exhibit significant dispersions. Our study reveals that hybridization in combination with an extended well-ordered adsorption structure of the π-conjugated organic molecules is a striking concept to receive and experimentally observe band formation at molecule/metal interfaces.
关键词： band formation,organic semiconductors,molecule/metal interfaces,hybridization,charge transport,density functional theory,angle-resolved two-photon photoemission
更新于2025-09-23 15:21:21