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Ligand-Assisted Formation of Graphene/Quantum Dot Monolayers with Improved Morphological and Electrical Properties
摘要： Hybrid nanomaterials based on graphene and PbS quantum dots (QDs) have demonstrated promising applications in optoelectronics. However, the formation of high-quality large-area hybrid films remains technologically challenging. Here, we demonstrate that ligand-assisted self-organization of covalently bonded PbS QDs and reduced graphene oxide (rGO) can be utilized for the formation of highly uniform monolayers. After the post-deposition ligand exchange, these films demonstrated high conductivity and photoresponse. The obtained films demonstrate a remarkable improvement in morphology and charge transport compared to those obtained by the spin-coating method. It is expected that these materials might find a range of applications in photovoltaics and optoelectronics.
关键词： graphene,self-assembly,charge transport,spectroscopy,monolayers,quantum dots
更新于2025-09-23 15:19:57
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[IEEE 2019 44th International Conference on Infrared, Millimeter, and Terahertz Waves (IRMMW-THz) - Paris, France (2019.9.1-2019.9.6)] 2019 44th International Conference on Infrared, Millimeter, and Terahertz Waves (IRMMW-THz) - THz excited state level spacing in encapsulated graphene quantum dots
摘要： We report a high-quality encapsulated graphene quantum dot that exhibits stable Coulomb diamonds and excited states with a spacing of 0.4 THz. We performed the first transport spectroscopy measurement under THz illumination of a large quantum dot. The photocurrent map allows to measure with high precision a non-linear chemical potential renormalization of the graphene electrodes via the interaction with the quantum dot states.
关键词： graphene quantum dots,THz,transport spectroscopy,chemical potential renormalization,photocurrent
更新于2025-09-11 14:15:04