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Quantum Dots Improve Photovoltaic Properties of Purple Membranes under Near-Infrared Excitation
摘要： Purple membrane (PMs), in which the photosensitive protein bacteriorhodopsin (bR) naturally occurs, have photovoltaic properties and are promising for optoelectronic applications. However, PMs cannot effectively absorb light in the NIR spectral region. Semiconductor quantum dots (QDs), which have high two-photon absorption cross-sections in the NIR region, can significantly improve the light sensitivity of PMs by means of F?rster resonance energy transfer (FRET) from QDs to bR inside PMs. The purpose of this study was to improve the photovoltaic properties of PMs by means of FRET from QDs to bR under NIR two-photon excitation. We made the QD-PM complexes and showed high FRET efficiency in them. Finally, we found that the current signal from the QD-PM material was higher than that in the case of PMs alone under NIR excitation. The obtained results clearly demonstrate improvement of the photovoltaic properties of PMs under NIR two-photon excitation due to the FRET from QDs to bR and show the prospect of designing new photosensitive bio-nanohybrid devices.
关键词： Near-Infrared Excitation,F?rster Resonance Energy Transfer,Purple Membranes,Photovoltaic Properties,Quantum Dots
更新于2025-09-11 14:15:04
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Study of Short-Term Photovoltaic Power Forecast Based on Error Calibration under Typical Climate Categories
摘要： With the increasing permeability of photovoltaic (PV) power production, the uncertainties and randomness of PV power have played a critical role in the operation and dispatch of the power grid and ampli?ed the abandon rate of PV power. Consequently, the accuracy of PV power forecast urgently needs to be improved. Based on the amplitude and ?uctuation characteristics of the PV power forecast error, a short-term PV output forecast method that considers the error calibration is proposed. Firstly, typical climate categories are de?ned to classify the historical PV power data. On the one hand, due to the non-negligible diversity of error amplitudes in different categories, the probability density distributions of relative error (RE) are generated for each category. Distribution ?tting is performed to simulate probability density function (PDF) curves, and the RE samples are drawn from the ?tted curves to obtain the sampling values of the RE. On the other hand, based on the ?uctuation characteristic of RE, the recent RE data are utilized to analyze the error ?uctuation conditions of the forecast points so as to obtain the compensation values of the RE. The compensation values are adopted to sequence the sampling values by choosing the sampling values closest to the compensation ones to be the ?tted values of the RE. On this basis, the ?tted values of the RE are employed to correct the forecast values of PV power and improve the forecast accuracy.
关键词： Latin hypercube sampling,error calibration,photovoltaic power forecast,nonparametric kernel density estimation,typical climate categories
更新于2025-09-11 14:15:04
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Solar Photovoltaic Panels Combined with Energy Storage in a Residential Building: An Economic Analysis
摘要： Renewable energy is a wide topic in environmental engineering and management science. Photovoltaic (PV) power has had great interest and growth in recent years. The energy produced by the PV system is intermittent and it depends on the weather conditions, presenting lower levels of production than other renewable resources (RESs). The economic feasibility of PV systems is linked typically to the share of self-consumption in a developed market and consequently, energy storage system (ESS) can be a solution to increase this share. This paper proposes an economic feasibility of residential lead-acid ESS combined with PV panels and the assumptions at which these systems become economically viable. The profitability analysis is conducted on the base of the Discounted Cash Flow (DCF) method and the index used is Net Present Value (NPV). The analysis evaluates several scenarios concerning a 3-kW plant located in a residential building in a PV developed market (Italy). It is determined by combinations of the following critical variables: levels of insolation, electricity purchase prices, electricity sales prices, investment costs of PV systems, specific tax deduction of PV systems, size of batteries, investment costs of ESS, lifetime of a battery, increases of self-consumption following the adoption of an ESS, and subsidies of ESS. Results show that the increase of the share of self-consumption is the main critical variable and consequently, the break-even point (BEP) analysis defines the case-studies in which the profitability is verified.
关键词： sensitivity analysis,photovoltaic,self-consumption,storage,economic analysis
更新于2025-09-11 14:15:04
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Photovoltaic Performance Enhancement of Perovskite Solar Cells Using Polyimide and Polyamic Acid as Additives
摘要： Poly(amic acid) (PAA) and polyimide (PI) can interact with Pb2+ and methylammonium halide by forming Lewis acid–base adducts and hydrogen bonds, respectively. These interactions can passivate perovskite (PVSK) defects and enhance PVSK solar cell (PSC) performance. Here, PAA and PI polymers were used as PSC additives by using p–i–n PSC [ITO/NiOx/CH3NH3PbI3/with or without PAA or PI/PC61BM/BCP/Ag], and PVSK’s interactions with PAA or PI were explored through X-ray photoelectron, UV–visible, photoluminescence (PL), and time-resolved PL spectroscopy. In additive-derived PVSKs, defects passivation increased PL intensity and carrier lifetime. Field emission scanning electron microscopy revealed increased grain size suggesting decreased grain boundary defects in PAA-derived PVSK. Moreover, 0.0497 mg/ml PAA/PVSK had high power conversion efficiency (14.16% ± 0.54% in control devices vs. 16.80% ± 0.63%; highest = 17.85%). PAA/PVSK displayed excellent shelf-life stability, with efficiency maintained at 16.57% ± 0.75% after storage in Ar-filled glovebox for >500 h.
关键词： Perovskite,photovoltaic,additive
更新于2025-09-11 14:15:04
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Highly efficient perovskite solar cells based on a Zn2SnO4 compact layer
摘要： In the present work, a new reflux condensation route has been developed for synthesizing Zn2SnO4 film, which was first used as a compact layer in a perovskite solar cell (PSC), and achieved an efficiency of 20.1%. The high efficiency of PSC could be contributed to the following: i) As a compact layer in a PSC, Zn2SnO4 exhibits high electron mobility and has an appropriate energy band structure, resulting in the efficient extraction of carriers and transport of electrons; ii) the surface of the FTO substrate is completely covered by a Zn2SnO4 compact layer, and the direct contact between a perovskite layer and FTO is prevented, leading to significantly efficiently suppression of charge recombination. Consequently, the cell consisting of a Zn2SnO4 compact layer exhibits excellent photovoltaic performance.
关键词： Zn2SnO4,photovoltaic property,compact layer,perovskite solar cells,charge recombination,energy band structure
更新于2025-09-11 14:15:04
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The role of NaF post-deposition treatment on the photovoltaic characteristics of semitransparent ultrathin Cu(In,Ga)Se <sub/>2</sub> solar cells prepared on indium-tin-oxide back contacts: a comparative study
摘要： Cu(In,Ga)Se2 (CIGSe) solar cells with absorber thicknesses of <500 nm are important for lowering the cost of photovoltaic (PV)-generated electricity. Moreover, ultrathin bifacial CIGSe solar cells can be prepared on indium-tin-oxide (ITO) back contacts (BCs). In contrast to Mo BCs, ITO BCs suppress the di?usion of Na from soda-lime glass (SLG) to the CIGSe absorber. Na present in the absorber is supposed to ameliorate the PV properties of CIGSe solar cells, but in the absence of Na or when the Na concentration is extremely low, the PV performance is expected to be poor. In this study, a NaF post-deposition treatment (PDT) was applied to a <500 nm thick semitrasparent CIGS absorber prepared by a 1-stage co-evaporation process. A detailed comparison is made between the CIGSe solar cell that underwent the NaF PDT (C–Na) and a reference CIGSe solar cell in which no Na was supplied from an external source (C0). All the PV parameters (i.e., the open-circuit voltage, short-circuit current density, ?ll factor, and e?ciency) of C–Na considerably improved compared with those of C0. To understand the factors that led to this improvement, the solar cells are analyzed by various characterization techniques, including JV measurements, external quantum e?ciency measurements, temperature-dependent measurements of the open-circuit voltage, capacitance–voltage measurements, drive level capacitance pro?lometry, and admittance spectroscopy. Furthermore, the reaction occurring at the CIGSe/ITO interface is investigated with transmission electron microscopy, and the implications of this reaction on the device performance are discussed.
关键词： ultrathin,solar cells,semitransparent,indium-tin-oxide back contacts,NaF post-deposition treatment,Cu(In,Ga)Se2,photovoltaic characteristics
更新于2025-09-11 14:15:04
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Photovoltaic, photo-impedance, and photo-capacitance effects of the flexible (111) BiFeO <sub/>3</sub> film
摘要： Ferroelectric polarization allows a depolarization electric field to separate electron-hole pairs excited by lights, and thus, the photovoltaic properties of ABO3-type films on a hard SrTiO3 or Si substrate have been extensively studied recently. However, there are a few reports on the photocapacitance and photoimpedance of these oxide films, especially on flexible substrates. In this work, the strong photovoltaic, giant photocapacitance, and photoimpedance effects were observed in the flexible (111) BiFeO3 films with natural downward polarization. The flexible mica/SrRuO3/BiFeO3/Au cells show a maximum photovoltaic efficiency at 150 °C, a 95.5% decrease in photoimpedance effects, and a 316% increase in photocapacitance effects under 405-nm-wavelength light illumination at 25 °C. Most importantly, these properties do not show obvious degradation when the device is bent to 3 mm radius for 104 times. This work is of vital importance for us to develop new flexible photoelectronic devices.
关键词： photo-capacitance,photovoltaic,flexible,photo-impedance,BiFeO3 film
更新于2025-09-11 14:15:04
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[IEEE 2019 Chinese Control And Decision Conference (CCDC) - Nanchang, China (2019.6.3-2019.6.5)] 2019 Chinese Control And Decision Conference (CCDC) - Event-triggered Dual-mode Control of Maximum Power Point Tracking for Photovoltaic Arrays
摘要： Photovoltaic power generation systems will switch between two situations: uniform illumination and local shadow. For maximum power point tracking (MPPT), the conventional strategy is often ef?cient in only one situation. But for both situations with switching, there face problems such that the tracking time may be too long or it may fall into the local maximum power point (LMPP). Aiming at these problems, in this paper, an event-triggered dual-mode control technology is proposed, which enables the system to work with high ef?ciency and high precision under both uniform illumination and local shadow. Under the uniform illumination, the maximum power point is tracked by the perturbation method (P&O), while in a local shaded environment, the current ?owing through the bypass diode acts as a trigger signal which enables Particle Swarm Optimization (PSO) to track the Global Maximum Power Point (GMPP). The simulation experiment by Matlab shows that in both the uniform illumination and local shadow, the algorithm of event-triggered dual-mode control is ef?cient in MPPT and has a fast and smooth transition between P&O and PSO, overcoming the problems of conventional strategy.
关键词： Event-triggered Dual-mode control,Photovoltaic power generation,Maximum power point tracking
更新于2025-09-11 14:15:04
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Systematic control of the rate of singlet fission within 6,13-diphenylpentacene aggregates with PbS quantum dot templates
摘要： Lead chalcogenide quantum dots (QDs) are promising acceptors for photovoltaic devices that harness the singlet fission (SF) mechanism. The rate of singlet fission of polyacenes in the presence of QDs is a critical parameter in determining the performance of such devices. The present study demonstrates that the rates of SF in a pentacene derivative, 6,13-dipenylpentacene (DPP), are modulated by forming coaggregates with PbS QDs in aqueous dispersions. PbS QDs generally accelerate SF within DPP aggregates, and the extent of acceleration depends on the size of the QD. The average rate of SF increases from 0.074 ps-1 for DPP-only aggregates to 0.37 ps-1 within DPP-D co-aggregates for QDs with radius 2.2 nm, whereas co-aggregation with the smallest (r = 1.6 nm) and largest (r = 2.7 nm) QDs we tried only slightly change the SF rate. The rate variation is associated with (i) the density of surface ligands, which is influenced by the faceting of the PbS surface, and (ii) the local dielectric constant for the DPP. To accelerate SF, the ligands should be dense enough to provide sufficient affinity for DPP aggregates and effectively perturb the perpendicular alignment of DPP monomers within aggregates to increase the intermolecular coupling that promotes SF, but should not be too dense so as to form a low dielectric environment that disfavors SF. The study suggests that it is critical to consider the influence of the microenvironment of QD surface on photophysical processes when fabricating QD/organic hybrid devices.
关键词： pentacene,photovoltaic devices,PbS,quantum dots,singlet fission
更新于2025-09-11 14:15:04
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[IEEE 2019 Chinese Control And Decision Conference (CCDC) - Nanchang, China (2019.6.3-2019.6.5)] 2019 Chinese Control And Decision Conference (CCDC) - Design and Simulation of Solar Photovoltaic Directional Tracking Device
摘要： With the rapid development of solar photovoltaic systems, the application and demand for solar tracking systems are growing accordingly. This paper, from an astronomical point of view, analyses movement of the sun and designs an integrated device for solar photovoltaic directional tracking based on the general formulas of solar declination, time angle, azimuth, and elevation angle. To improve tracking accuracy and efficiency, the device is designed by using a double-degree-of-freedom tracking system, so that it can track the sun in both horizontal and vertical directions. Besides, a hybrid tracking mode is applied to achieve accurate tracking of the sun movement, in which the solar trajectory tracking is used as the primary mode, while the photoelectric monitoring is taken as a supplementary, to improve the accuracy and stability of the algorithm. The results from the simulation carried out by Proteus software reveals that the device as well as the control system both operate in a stable and reliable manner, during which, the solar panel is perpendicular to the sun's direct rays within an acceptable range of deviation, realizing the automatic tracking of the sun's rays all the time, which significantly improves the receiving efficiency of solar energy.
关键词： Solar Tracking,Photovoltaic system,Solar trajectory tracking,Directional tracking device
更新于2025-09-11 14:15:04