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Complex-conjugate Pole-residue Pair-Based FDTD Method for Assessing Ultrafast Transient Plasmonic Near Field

DOI:10.1007/s11468-019-01057-x 期刊:Plasmonics 出版年份:2019 更新时间:2025-09-11 14:15:04
摘要: The study of the optical properties of plasmonic nanostructures in the stationary regime has greatly benefited from the development of numerical methods, among which Finite Difference Time Domain (FDTD) is popular. In contrast, the use of these numerical tools for assessing the transient plasmonic optical response triggered by ultrashort laser pulses is hampered by the difficulty to address small variations of the material optical properties with reasonable computational time. Yet, many of the developments based on this ultrashort response rely on the dynamics of the near-field topography around the nanostructures. In this article, we present a way to bridge this gap with the complex-conjugate pole-residue pair (CCPRP) approach. A CCPRP-based FDTD simulator has been developed. First, a simple methodology to check the end-to-end accuracy of the FDTD simulation is provided. Then, in conjunction with a three-temperature model, the approach enables us to calculate the ultrafast transient near field inside and around a gold nanoparticle (AuNP) upon absorption of a subpicosecond laser pulse. The transient variation of the field intensity inside and around the AuNP is compared with the one determined by the Mie theory. The dependence of the transient field intensity on the distance away from the nanoparticle surface and on the delay time after laser pulse absorption is finally analyzed.
作者: Tadele Orbula Otomalo,Fabrice Mayran de Chamisso,Bruno Palpant
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To bridge the gap in assessing the transient plasmonic optical response triggered by ultrashort laser pulses by developing a complex-conjugate pole-residue pair (CCPRP) approach for FDTD simulation.

The CCPRP-based FDTD method, combined with the 3TM, effectively models the ultrafast transient variation of the near-field intensity enhancement in and around a gold nanoparticle. The method's accuracy was validated, and it was shown to be suitable for investigating phenomena triggered by ultrashort laser pulses related to near-field enhancement in plasmonic nanostructures.

The approach is limited to a 'slow' variation of the dielectric function with respect to the time scale of the field oscillation, suitable for perturbative modeling. The study also notes discrepancies between FDTD calculations and Mie theory, possibly due to the geometrical representation of the AuNP in simulations.

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