研究目的
Investigating the tailoring of second-harmonic generation in plasmonic radial trimers using cylindrical vector beams.
研究成果
The work demonstrates a new route to manipulate the efficiency of second-harmonic generation on the nanoscale using novel assemblies of nanostructures and unconventional optical beams.
研究不足
Possible imperfections in the real trimers and cylindrical vector beams may affect the experimental results.
1:Experimental Design and Method Selection:
The study involved fabricating plasmonic trimers on a cover glass using electron-beam lithography and studying them using a custom-built point-scanning SHG microscope.
2:Sample Selection and Data Sources:
The trimers consisted of three equal-sized gold nanobars, with their spatial distribution designed to match the fundamental excitation wavelength used in the SHG measurements.
3:List of Experimental Equipment and Materials:
A femtosecond laser (1060 nm, 140 fs, 80 MHz, 1 mW), a microscope objective (NA =
4:8), a stage-scanner, a cooled photomultiplier tube, and a polarization mode converter were used. Experimental Procedures and Operational Workflow:
The trimers were illuminated symmetrically by cylindrical vector beams, and SHG signals were measured.
5:Data Analysis Methods:
Numerical calculations based on the boundary element method were used to analyze the results.
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