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Solution‐Processed Laminated Perovskite Layers for High‐Performance Solar Cells

DOI:10.1002/adfm.201903330 期刊:Advanced Functional Materials 出版年份:2019 更新时间:2025-09-19 17:13:59
摘要: In this study, the combined effect of dissolved oxygen (DO) and COD/N on nitrogen (N) removal as well as the corresponding mechanisms were investigated in aerated constructed wetlands (CWs). At each investigated COD/N level, the ammonium removal efficiency increased as DO concentration increased. However, the highest total N removal efficiency occurred at different DO concentration at each COD/N level. The results of functional gene analysis and cyclic N profile studies indicated that DO supply and COD/N influence the N removal performance, which is not only exert a direct effect on nitrification-denitrification process, but also change N removal pathway in intermittent aerated CWs. At a relatively high influent COD/N of 20, the simultaneous nitrification and denitrification (SND) via nitrite was almost the exclusive N removal pathway at all investigated DO concentration. With the decrease of COD/N from 20 to 2 at DO of ~1.8, ~3.5 and ~6.0 mg/L, SND efficiency all decreased, however, its decreasing rate was much higher at relatively high DO level of ~6.0 mg/L than that at DO levels of ~1.8 and ~3.5 mg/L. In comparison, a simultaneously partial nitrification, anammox and denitrification was established at DO of ~0.8 mg/L along with reducing influent COD/N.
作者: Jie Wang,Jie Hou,Ling Xia,Zhiming Jia,Xugang He,Dapeng Li,Yiyong Zhou
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Investigating the combined effect of dissolved oxygen (DO) and COD/N on nitrogen (N) removal as well as the corresponding mechanisms in aerated constructed wetlands (CWs).

The study proved that DO supply and influent COD/N ratio had a combined effect on N removal through regulating the N removal pathway in intermittent aeration CWs. SND was dominant N removal pathway in a broad range of DO and COD/N conditions, while anammox-dominated SNAD could be dominant only at low DO along with low COD/N levels. Enhancing DO supply could improve ammonium removal efficiency at each investigated influent COD/N levels. However, the optimal DO supply for total N removal should be adjusted according to the influent COD/N ratio.

The major limitation of this study is that the major microbial nitrogen removal pathway under various DO and influent COD/N levels was concluded from circumstantial evidences, such as the characteristics of wastewater, transformation of nitrogen and abundance of functional genes involving the cycling of N. Quantification of active genes using mRNA-based technology and batch activity tests could provide more precise results.

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