摘要： This multidisciplinary paper reports on a research application-led study for predicting atmospheric attenuation, and tries to bridge the knowledge gap between applied engineering and atmospheric sciences. As a useful comparative baseline, this paper focuses specifically on atmospheric attenuation under pristine conditions, over the extended terahertz spectrum. Three well-known simulation software packages (‘HITRAN on the Web’, MODTRAN R(cid:13)4, and LBLRTM) are compared and contrasted. Techniques used for modeling atmospheric attenuation have been applied to investigate the resilience of (ultra-)wide fractional bandwidth applications to the effects of molecular absorption. Two extreme modeling scenarios are investigated: horizontal path links at sea level and Earth-space path links. It is shown by example that a basic software package (‘HITRAN on the Web’) can give good predictions with the former, whereas sophisticated simulation software (LBLRTM) is required for the latter. Finally, with molecular emission included, carrier-to-noise ratio fade margins can be calculated for the effects of line broadening due to changes in macroscopic atmospheric conditions with sub-1-THz ultra-narrow fractional bandwidth applications. Outdoors can be far from pristine, with additional atmospheric contributions only briefly introduced here; further discussion is beyond the scope of this paper, but relevant references have been cited.