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Passively Q-switched near-infrared lasers with bismuthene quantum dots as the saturable absorber

DOI:10.1016/j.optlastec.2020.106219 期刊:Optics & Laser Technology 出版年份:2020 更新时间:2025-09-23 15:19:57
摘要: Bismuthene quantum dots (Bi-QDs) were synthesized via the liquid phase exfoliation (LPE) method for the passive Q-switching operation in near-infrared (NIR) region. The nonlinear optical properties of the prepared Bi-QDs were investigated by the open-aperture Z-scan technology. The modulation depths were 18.1% and 5.1% at 1.06 and 1.34 μm, respectively. Based on the Bi-QDs saturable absorber, passively Q-switched Nd:GdVO4 lasers operating at 4F3/2 → 2I11/2 and 4F3/2 → 2I13/2 transitions were demonstrated, showing the wideband optical modulation in NIR regime. For the 4F3/2 → 2I13/2 transition lasing at 1.34 μm, the shortest pulse duration of 155 ns was obtained with a repetition rate of 457 kHz. With respect to the 4F3/2 → 2I11/2 transition at 1.06 μm, the minimum pulse duration was 150 ns with a repetition rate of 424 kHz, leading to a single pulse energy of 261 nJ and a peak power of 1.68 W. In addition, the ground state absorption cross section and the excited state absorption cross section of Bi-QDs were also investigated for the ?rst time. The impact of the excited state lifetime on the output parameters was numerically stimulated by the coupled rate equations. Our work con-?rmed that the trap state in Bi-QDs played an important role in the pulse generation mechanism.
作者: Li Dong,Weichun Huang,Hongwei Chu,Guiqiu Li,Han Zhang,Dechun Li,Ying Li,Yunzheng Wang,Shengzhi Zhao
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To investigate the nonlinear optical properties of bismuthene quantum dots (Bi-QDs) and their application as saturable absorbers in passively Q-switched near-infrared (NIR) lasers.

The study demonstrated that Bi-QDs synthesized via the LPE method exhibit significant nonlinear optical properties, making them suitable as saturable absorbers in passively Q-switched NIR lasers. The shortest pulse durations of 150 ns and 155 ns were achieved at 1.06 and 1.34 μm, respectively. The ground state and excited state absorption cross sections of Bi-QDs were calculated for the first time, and the impact of the excited state lifetime on laser performance was numerically simulated. The findings confirm the potential of Bi-QDs for applications in ultrafast photonics.

The study focused on the nonlinear optical properties and application of Bi-QDs as saturable absorbers in NIR lasers. The limitations include the need for further optimization of Bi-QDs quality and laser cavity design to achieve shorter pulse durations and higher peak powers.

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