研究目的
To present a novel 11 eV tr-ARPES setup that achieves high energy and time resolutions at high repetition rates for studying the non-equilibrium band structure of solids.
研究成果
The 11 eV tr-ARPES setup achieves unprecedented energy and time resolutions, enabling high-resolution, momentum-selective non-equilibrium studies of the band structure across a wide range of the Brillouin zone. The setup's high repetition rates and tunability make it a powerful tool for studying the nonequilibrium band structure on sub-picosecond timescales.
研究不足
The energy resolution is slightly limited at the widest slit opening due to instrument limitations. The time resolution is lower than the pulse width of the laser output due to dispersive optical elements and non-collinear propagation of pump and probe beams.
1:Experimental Design and Method Selection:
The setup uses a series of two harmonic generation stages to produce bright 11 eV laser pulses at high repetition rates.
2:Sample Selection and Data Sources:
Measurements were taken on n-doped Bi2Se3 single crystals and ErTe3 single crystals.
3:List of Experimental Equipment and Materials:
Includes a 1038 nm, 190 fs Yb:KGW amplifier laser, nonlinear crystals, a hollow-core fiber filled with xenon gas, and a custom-built monochromator.
4:Experimental Procedures and Operational Workflow:
The 11 eV beam is generated and then directed through a monochromator to filter out unwanted wavelengths before focusing onto the sample in the ARPES chamber.
5:Data Analysis Methods:
Energy distribution curves (EDCs) were fitted using a Gaussian-convoluted Fermi–Dirac distribution to determine energy resolution.
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Yb:KGW amplifier laser
PHAROS
Light Conversion
Generates the initial laser pulses for the harmonic generation process.
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Optical parametric amplifier
ORPHEUS
Light Conversion
Generates tunable wavelengths from the ultraviolet to near-infrared range.
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Third harmonic generator
HIRO
Light Conversion
Generates the third harmonic of the initial laser pulses.
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Monochromator
OP-XCT
McPherson Inc.
Filters out unwanted wavelengths and transmits the 9ω component to the ARPES chamber.
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CCD
Newton
Andor
Diagnoses the overall intensity and fiber propagation mode of the 11 eV beam.
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Photodiode
AXUV 100 G
Opto Diode Corp.
Measures the 11 eV flux accurately.
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Hollow-core fiber
XUUS
KM Labs
Filled with xenon gas for another third harmonic generation process.
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Time-of-flight electron analyzer
ARTOF 10K
Scienta Omicron
Measures the energy and momentum of photoelectrons.
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