研究目的
Preparation and characterization of visible-enhanced PbI2/MgO/Si heterojunction photodetector by pulsed laser deposition technique.
研究成果
The study successfully prepared high visible responsivity nanostructured PbI2/MgO/Si heterojunction photodetector by PLD method without using post annealing. The presence of MgO buffer layer between PbI2 film and silicon substrate improved the junction characteristics. The maximum responsivity of 0.88A/W at 410nm was obtained at a preparation temperature of 45°C. The photodetector can be used efficiently for detecting visible weak signals.
研究不足
The study does not mention the long-term stability or durability of the photodetectors under continuous operation. The effect of environmental factors on the performance of the photodetectors was not investigated.
1:Experimental Design and Method Selection:
The study used pulsed laser deposition (PLD) technique for fabricating p-PbI2/MgO/n-Si photodetectors. The structural, optical, and morphological properties of the films were investigated using XRD, UV-Vis absorption, and SEM.
2:Sample Selection and Data Sources:
N-type silicon substrates of (111) orientation were used. The substrates were cleaned and etched with diluted hydrofluoric acid to remove the surface oxide.
3:List of Experimental Equipment and Materials:
A lab-assembled PLD system, Nd: YAG laser, laser interferometer system, X-ray diffractometer (XRD-6000, Shimadzu), scanning electron microscope SEM (T-scan Vega III Czech), double beam UV-Vis spectrophotometer (Metratech SP 8001), and LCR meter were used.
4:Experimental Procedures and Operational Workflow:
MgO thin film was deposited on quartz and silicon substrates at 100°C by PLD. PbI2 thin film was then deposited on MgO film by PLD at temperatures (25, 45, 65, and 100)°C. The ohmic contacts were established by depositing In on the PbI2 film and Al on the back side of silicon substrate.
5:Data Analysis Methods:
The current-voltage and capacitance-voltage characteristics were measured at room temperature. The responsivity of the photodetector was measured using a calibrated Jobin Yvon monochromator.
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