研究目的
Investigating the emergence of point defect states in a plasmonic crystal and their relationship with the band structure of the crystal.
研究成果
The relationship between the band structure of the PlBG and the defect mode was revealed, giving the formation model of the defect mode. The energy level of the band-edge mode lying at the highest level of the first band is elevated by introduction of the flat area, resulting in formation of the modified mode within the band gap energy range. The defect mode is already formed in the two rings structure, which coincides with emergence of periodicity of the ring structure.
研究不足
The study is limited by the technical constraints of EELS measurements, including the need for high spatial and momentum resolution. The applicability of far-field techniques is limited above the second band, and defect modes are expected to be nonradiative if their energy levels lie within the first band gap.
1:Experimental Design and Method Selection:
The study combined spatially-resolved spectroscopy and momentum-resolved spectroscopy of EELS to investigate the relationship between the band structure of the PlBG and the defect mode.
2:Sample Selection and Data Sources:
Plasmonic crystals with a triangular lattice were fabricated using e-beam lithography, and point defects were introduced deliberately.
3:List of Experimental Equipment and Materials:
A monochromated scanning transmission electron microscope (STEM) Nion Hermes 200-S was used for EELS measurements.
4:Experimental Procedures and Operational Workflow:
Spatially-resolved EELS was performed to observe localized modes at point defects, and momentum-resolved EELS was used to measure the band dispersion relation of the bulk crystal.
5:Data Analysis Methods:
The experimental results were compared with FDTD simulations to confirm the energy position of the band gap and the formation mechanism of the defect mode.
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