研究目的
Investigating the durable and stable UV–Vis perovskite photodetectors based on CH3NH3PbI3 crystals synthesized via a solvothermal method.
研究成果
The durable and stable UV–Vis perovskite photodetectors based on CH3NH3PbI3 crystals synthesized via a solvothermal method exhibited high performance, including a high on/off photocurrent ratio, fast response and decay times, and excellent durability and stability, making them potentially applicable for practical applications.
研究不足
The study's limitations include the potential for surface defects in the perovskite thin films and the sensitivity of the device's performance to the interface states between Au and CH3NH3PbI3.
1:Experimental Design and Method Selection:
The study involved the synthesis of CH3NH3PbI3 crystals via a solvothermal method and the fabrication of photodetectors with a coplanar MSM IDT patterned Au electrode configuration.
2:Sample Selection and Data Sources:
The samples were prepared using Pb(Ac)2·3H2O, HI, isopropanol, and methylamine solution.
3:List of Experimental Equipment and Materials:
Instruments included X-ray diffraction (XRD), field-emission scanning electron microscope (FE-SEM), photoluminescence (PL) spectrophotometer, UV–Vis diffuse reflectance spectroscopy (DRS), and Keithley 4200 semiconductor device analyzer.
4:Experimental Procedures and Operational Workflow:
The synthesis involved dissolving Pb(Ac)2·3H2O in HI, adding isopropanol and methylamine solution, and maintaining at 150 °C for 4 h. The photodetectors were fabricated by spin-coating the precursor solutions on IDT patterned Au electrodes.
5:Data Analysis Methods:
The performance of the photodetectors was analyzed using I–V characteristics, transient photo-response characteristics, and responsivity calculations.
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