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Evidence of Pure Spin-Current Generated by Spin Pumping in Interface Localized States in Hybrid Metal-Silicon-Metal Vertical Structures

DOI:10.1021/acs.nanolett.8b03386 期刊:Nano Letters 出版年份:2018 更新时间:2025-09-09 09:28:46
摘要: Due to the difficulty to grow high quality semiconductors on ferromagnetic metals, the study of spin diffusion transport in Si was only limited to lateral geometry devices. In this work, by using ultra-high vacuum wafer-bonding technique, we have successfully fabricated metal-semiconductor-metal CoFeB/MgO/Si/Pt vertical structures. We hereby demonstrate pure spin-current injection and transport in the perpendicular current flow geometry over a distance larger than 2μm in n-type Si at room temperature. In those experiments, a pure propagating spin-current is generated via ferromagnetic resonance spin-pumping and converted into a measurable voltage by using the inverse spin-Hall effect occurring in the top Pt layer. A systematic study by varying both Si and MgO thicknesses reveals the important role played by the localized states at the MgO/Si interface for the spin-current generation. Proximity effects involving indirect exchange interactions between the ferromagnet and the MgO/Si interface states appears to be a prerequisite to establish the necessary out-of-equilibrium spin-population in Si under the spin-pumping action.
作者: Carolina Cerqueira,Jianyin Qin,Huong Dang,Abdelhak Djeffal,Jean Christophe LE BRETON,Michel Hehn,Juan Carlos Rojas Sanchez,Xavier Devaux,Stéphane Suire,Sylvie Migot,Philippe Schieffer,Jean-Georges Mussot,Piotr #aczkowski,Abdelmadjid Anane,Sebastien Petit-Watelot,Mathieu Stoffel,Stéphane Mangin,Zhi Liu,Buwen Cheng,Xiufeng Han,Henri Jaffres,Jean-Marie George,Yuan Lu
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To demonstrate pure spin-current injection and transport in the perpendicular current flow geometry over a distance larger than 2μm in n-type Si at room temperature using metal-semiconductor-metal CoFeB/MgO/Si/Pt vertical structures fabricated by ultra-high vacuum wafer-bonding technique.

The study successfully demonstrates efficient spin-current injection and transport at room temperature in CoFeB/MgO/Si/Pt vertical devices, highlighting the significant role of localized states at the MgO/Si interface in spin-current generation. The spin-diffusion length in n-Si is determined to be 2.0±0.3μm at room temperature, indicating the potential for semiconductor spintronics applications.

The study is limited by the difficulty in growing high quality semiconductors on ferromagnetic metals, which restricts the investigation to lateral geometry devices without the use of wafer-bonding technique. Additionally, the role of localized states at the MgO/Si interface and their impact on spin-current generation requires further theoretical and experimental exploration.

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